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  • 1
    ISSN: 1432-0649
    Keywords: 42.65 ; 68.35
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract A wavelength-dependence study of surface second-harmonic generation from Si(111) is presented. Femtosecond laser pulses tuned from 430 nm to 710 nm were used to probe the dispersion characteristics of the nonlinear response from the surface in the vicinity of bulk absorption. Changes in the rotational symmetry and in the phase of the generated second-harmonic signal were observed. An explanation of the observed changes is given based on a simple anharmonic oscillator model [1]
    Type of Medium: Electronic Resource
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  • 2
    ISSN: 1432-0630
    Keywords: 42.65 ; 68.35
    Source: Springer Online Journal Archives 1860-2000
    Topics: Mechanical Engineering, Materials Science, Production Engineering, Mining and Metallurgy, Traffic Engineering, Precision Mechanics , Physics
    Notes: Abstract Direct measurement of the phase of the surface nonlinear susceptibility is based on the interference of nonlinear optical signals. Up to now, this has not been possible for Second-Harmonic Generation (SHG) in geometries such as Total Internal Reflection (TIR) due to the refractive dispersion of harmonic and fundamental light created in TIR. We demonstrate two schemes which enable us to overcome this dispersion, leading to interference between two second-harmonic signals generated consecutively by the same laser. The advantages and limitations of the two approaches are discussed. We use this technique to check the theoretical predictions for the nonlinear Fresnel factors for SHG in the TIR geometry.
    Type of Medium: Electronic Resource
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