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  • Organic Chemistry  (2)
  • Addiction  (1)
  • Bissilylamines  (1)
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  • 1
    Digitale Medien
    Digitale Medien
    Nicotine addiction: a re-analysis of the arguments (1992)
    Springer
    Psychopharmacology 108 (1992), S. 408-410 
    Details
    ISSN: 1432-2072
    Schlagwort(e): Smoking ; Nicotine ; Dependence ; Addiction
    Quelle: Springer Online Journal Archives 1860-2000
    Thema: Medizin
    Notizen: Abstract This paper evaluates the arguments put forward by Robinson and Pritchard (R&P, this volume) that the conclusions of the US Surgeon General (USDHHS 1988) that nicotine is addictive were ill founded. R&P state that nicotine does not cause intoxication, that many smokers do not exhibit compulsive use, that nicotine is not a euphoriant, that nicotine is a weak reinforcer in other species, that non-pharmacological aspects of smoking are important and that negative affect control accounts for more of the variance in questionnaire measures of smoking motives than does habit. This paper points out that intoxication and a euphoriant effect are not normally considered to be central to dependence potential, that no addictive drug results in compulsive use in all users in all situations, that animals do reliably self-administer nicotine, that evidence concerning the apparent importance of non-pharmacological components of smoking do not diminish the importance of pharmacological aspects and that “variance accounted for” of self-report measures of smoking motivation do not bear on the issue of the importance of those motives. The paper concludes with a summary of the essence of the argument that cigarettes are addictive and that nicotine is the primary focus of that addiction.
    Materialart: Digitale Medien
    URL: http://dx.doi.org/10.1007/BF02247413
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  • 2
    Digitale Medien
    Digitale Medien
    Synthetic and Structural Studies of 1-Sila-2,5-diaryltetrazenes (1997)
    Weinheim : Wiley-Blackwell
    Berichte der deutschen chemischen Gesellschaft 130 (1997), S. 1579-1583 
    Details
    ISSN: 0009-2940
    Schlagwort(e): Silatetrazenes ; Nitrogen-silicon ring systems ; Bissilylamines ; Silicon-29 solid state NMR ; Aryl azides ; Chemistry ; Inorganic Chemistry
    Quelle: Wiley InterScience Backfile Collection 1832-2000
    Thema: Chemie und Pharmazie
    Notizen: The reaction between aryl azides and lithiated aryl amines leads to tetrazenes 3 and 9 which contain a chain of four nitrogen atoms. Reaction with different halosilanes gives the cyclic silatetrazenes 10, 12, and 15 where substitutents on the silicon vary form alkyl to hydrogen and chlorine atoms. The structures of 10, 12, and 15 in the solid state are reported. Variation of the solvent and the Lewis acidity of the halosilane influence the ratio of silatetrazene to side products, bissilyated amines. These effects are studied for different halosilanes.
    Zusätzliches Material: 2 Tab.
    Materialart: Digitale Medien
    URL: http://dx.doi.org/10.1002/cber.19971301105
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  • 3
    Digitale Medien
    Digitale Medien
    Photoinitiation of vinyl polymerization by polysilanes (1987)
    New York, NY [u.a.] : Wiley-Blackwell
    Applied Organometallic Chemistry 1 (1987), S. 7-14 
    Details
    ISSN: 0268-2605
    Schlagwort(e): Polysilanes ; photoinitiation ; polymerisation ; vinyl monomers ; thin films ; photolysis ; Chemistry ; Organic Chemistry
    Quelle: Wiley InterScience Backfile Collection 1832-2000
    Thema: Chemie und Pharmazie
    Notizen: Polysilanes were found to photoinitiate the polymerization of a variety of vinyl monomers including methyl methacrylate, styrene, ethyl acrylate and acrylic acid. Polymerization initiated by polysilane photolysis is rather insensitive to oxygen inhibition, which may make it especially suitable for polymerization of thin films. The initiation efficiency of poly(phenylmethylsilylene) in styrene was determined from dilatometry data to be 1 × 10-3. This rather low efficiency is counterbalanced by the very high extinction coefficient of polysilane polymers, ca. 4-8 × 103 per silicon atom. Possible reasons for the low initiation efficiency and reduced oxygen inhibition of polysilane photoinitiators are discussed.
    Zusätzliches Material: 4 Ill.
    Materialart: Digitale Medien
    URL: http://dx.doi.org/10.1002/aoc.590010103
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  • 4
    Digitale Medien
    Digitale Medien
    Organosilicon polymers with alternating σ- and π-conjugated systems (1994)
    New York, NY [u.a.] : Wiley-Blackwell
    Applied Organometallic Chemistry 8 (1994), S. 423-430 
    Details
    ISSN: 0268-2605
    Schlagwort(e): organosilicon ; polymers ; semiconducting ; Chemistry ; Organic Chemistry
    Quelle: Wiley InterScience Backfile Collection 1832-2000
    Thema: Chemie und Pharmazie
    Notizen: A series of organosilicon polymers containing polysilane and diethynylaryl units along the polymer backbone were synthesized and examined with respect to their optical absorptions. The results indicate that delocalization takes place through the σ-π conjugated system. Lengthening of π-conjugation leads to lower excitation energies while nearly identical UV-vis spectra are observed with increased Si-Si chain length. Introducing a thiophene unit into the π-system instead of a benzene unit leads to a bathochromic shift reflecting greater σ-π delocalization. The polymers undergo photodegradation, probably via cleavage of the Si-Si bonds, and thermal crosslinking by reaction at the C≡C triple bonds. When doped with iodine, these polymers become semiconducting with conductivity of the order of 10-4 S cm-1.
    Zusätzliches Material: 7 Ill.
    Materialart: Digitale Medien
    URL: http://dx.doi.org/10.1002/aoc.590080417
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