ISSN:
1435-1528
Keywords:
Viscoelastic instability
;
secondary flow visualization
;
Taylor-Couette
;
Boger fluids
Source:
Springer Online Journal Archives 1860-2000
Topics:
Chemistry and Pharmacology
,
Physics
Notes:
Abstract Flow visualization is performed on an elastically-dominated instability in several similar Boger fluids in Taylor-Couette flow. The onset and evolution of secondary flow are observed over a range of shear rates using reflective mica platelet seeding. Sequences of ambiently and sheet-illuminated images were digitally processed. Rotation of the inner cylinder was ramped from rest to its final value over a time on the order of a polymer relaxation time. Dilute solutions of high molecular weight polyisobutylene in oligomeric polybutene manifest a flow transition at a Deborah number, De s = λ s γ ≈ 1.5 with a Taylor number of 0.00022 in a cell with dimensionless gap ratio δ = 0.0963. At this transition, simple azimuthal shearing is replaced by steady, roughly square, axisymmetric counter-rotating vortices grossly similar to the well-known Taylor vortex flow that is observed at De s = 0, Ta = 3612. At De s = 3.75, Ta = 0.0014, an axisymmetric oscillatory secondary flow develops initially but is replaced by the steady vortices. At De s = 7.5, Ta = 0.0054, the oscillatory and vortex flow coexist and possess an irregular cellular cross-section. A wide span of growth rates is observed: the ratio of onset to polymer relaxation time ranges from 170000 at De s = 1.5 to O(10) at De s 〉 5. The role of inertia was explored through changing the solvent viscosity. A transition similar to the one that occurs at De s = 3.75, Ta = 0.0014, from the base azimuthal shearing flow to axisymmetric vortices, was also observed with a much lower viscosity fluid at De s = 3.3, Ta = 74.
Type of Medium:
Electronic Resource
URL:
http://dx.doi.org/10.1007/BF00398434
Permalink
