ISSN:
1349-9432
Schlagwort(e):
third-order nonlinear optical response
;
second hyperpolarizability
;
open-shell systems
;
iso-electronic systems
;
charged radical
Quelle:
Springer Online Journal Archives 1860-2000
Thema:
Physik
Notizen:
Abstract We study the second hyperpolarizabilities (ɣ) for anion, neutral and cation radicals and find that magnitudes of ɣ (| ɣ |) of the radicals are sensitively influenced by features of each charged state. It is also found that electron-correlation dependence of ɣ could be related to the resonance structure contributing to the ground state of the molecules.
Materialart:
Digitale Medien
URL:
http://dx.doi.org/10.1007/s10043-999-0237-7
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