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  • 1
    Electronic Resource
    Electronic Resource
    Surface laser damage thresholds determined by photoacoustic deflection (1988)
    Woodbury, NY : American Institute of Physics (AIP)
    Applied Physics Letters 53 (1988), S. 2005-2007 
    Details
    ISSN: 1077-3118
    Source: AIP Digital Archive
    Topics: Physics
    Notes: The technique of intensity dependent photoacoustic probe beam deflection has been applied to the determination of surface damage thresholds. We take advantage of an unambiguous correlation between the degree of laser damage and the energy in the generated acoustic pulse. The high sensitivity of this method, cross checked by measuring scatter losses in reflection, is independent of any surface optical properties. As an example for optical materials, damage thresholds for MgF2 and CaF2 have been determined to be about 1.4 GW/cm2 , and for LiF to be about 0.2 GW/cm2 .
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1063/1.100491
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    Paper (German National Licenses)
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  • 2
    Electronic Resource
    Electronic Resource
    REMPI as a tool for studies of OH radicals in catalytic reactions (1997)
    Springer
    Applied physics 64 (1997), S. 573-578 
    Details
    ISSN: 1432-0649
    Keywords: PACS: 33.80K, 07.75, 82.65J
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: 2 +½ O2→H2O on polycrystalline Pt foils has been studied by detection of desorbing OH radicals using the Resonance Enhanced Multiphoton Ionization, REMPI, technique. The measurements were performed at catalyst temperatures of 1000–1400 K and a total pressure below 10-4 mbar. The studies of OH desorption by REMPI were achieved using a two-photon excitation D2Σ-–X2Π (1–0), followed by one-photon ionization. The ions were detected in a time-of-flight mass spectrometer, TOF-MS, in order to avoid interference from non-resonantly ionized molecules. By applying TOF-MS, a simultaneous non-resonant ionization and detection of H2, O2 and H2O was achieved. Recorded REMPI spectra were compared with spectra simulated using known molecular constants. The kinetics of the reaction derived from the measurements were compared with what was obtained in earlier LIF detection of OH, performed at higher total reactant pressure using the A–X transition. REMPI TOF-MS is shown to be a complement to LIF for reaction studies below 5×10-4 mbar total pressure, where LIF is too insensitive for quantification. The reaction kinetics was found to be in agreement with a theoretic model and previous LIF studies.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/s003400050217
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    Paper (German National Licenses)
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  • 3
    Electronic Resource
    Electronic Resource
    Adsorption of oxygen and hydrogen on Pt(111) studied with second-harmonic generation (1995)
    Springer
    Applied physics 60 (1995), S. 209-215 
    Details
    ISSN: 1432-0630
    Keywords: 68.35 ; 82.20 ; 42.65
    Source: Springer Online Journal Archives 1860-2000
    Topics: Mechanical Engineering, Materials Science, Production Engineering, Mining and Metallurgy, Traffic Engineering, Precision Mechanics , Physics
    Notes: Abstract The adsorption of oxygen and hydrogen on a Pt(111) surface has been studied with phase-sensitive Second-Harmonic Generation (SHG) signal detection. The SHG-signal change measured with p-in, p-out polarization during the adsorption of oxygen and hydrogen was found to be different in amplitude and phase for the two adsorbates. At the wavelength used (1064 nm), only a localized interaction between adsorbate and substrate is seen, leading to a linear dependence of the susceptibility on the coverage. Sticking coefficients,sθ, and their coverage dependence were determined. For hydrogen, a linear decrease insθ with coverage was found; the initial sticking coefficient beings 0=0.06 at a temperature ofT=130 K. For oxygen,sθ whows a quadratic decrease with coverage, strongly dependent on temperature, withs 0=0.05 atT=350 K. A method based on these results is proposed, which would allow the determination of adsorbate coverages of coadsorption systems with SHG using phase-sensitive signal detection.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01538248
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  • 4
    Electronic Resource
    Electronic Resource
    The role of defects in laser surface damage thresholds of fluoride crystals (1989)
    Springer
    Applied physics 49 (1989), S. 199-204 
    Details
    ISSN: 1432-0630
    Keywords: 42.85Fe ; 61.80Ba ; 42.20Ji
    Source: Springer Online Journal Archives 1860-2000
    Topics: Mechanical Engineering, Materials Science, Production Engineering, Mining and Metallurgy, Traffic Engineering, Precision Mechanics , Physics
    Notes: Abstract The energy of the acoustic pulse generated by laser-surface interactions and measured by probe beam deflection was used to investigate laser surface damage thresholds of fluoride crystals with optical quality. It was found that damage thresholds decrease with increasing density of surface states. The defect density also controls the energy absorption mechanism: for surfaces with few defects, like polished MgF2 and CaF2, avalanche breakdown occurs at above 1 GW/cm2, whereas for materials with lower damage thresholds, such as LiF, BaF2, and roughened or incubated surfaces of CaF2, multiphoton absorption across the band gap is observed.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00616299
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    Paper (German National Licenses)
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