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Kinetics and mechanism of the hydrogenation of cyclohexene (1975)

Hendrikse, J. L. ; Kaspersma, J. H. ; Coenen, J. W. E.

New York, NY : Wiley-Blackwell

International Journal of Chemical Kinetics 7 (1975), S. 557-574

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Details

ISSN: 0538-8066

Keywords: Chemistry ; Physical Chemistry

Source: Wiley InterScience Backfile Collection 1832-2000

Topics: Chemistry and Pharmacology

Notes: The rate of hydrogenation of cyclohexene, catalyzed by CoH3(PPh3)3, has been measured under various conditions and, based on these data, a mechanism has been postulated. For the individual steps of the mechanism enthalpy and entropy differences have been determined. The interpretation of these parameters gives evidence for a more detailed mechanism, in which solvent molecules play an important part as “stand-in” for ligands, dissociated from the catalyst species.

Additional Material: 8 Ill.

Type of Medium: Electronic Resource

URL: http://dx.doi.org/10.1002/kin.550070407

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