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  • 1
    Electronic Resource
    Electronic Resource
    Palo Alto, Calif. : Annual Reviews
    Annual Review of Nuclear and Particle Science 50 (2000), S. 411-479 
    ISSN: 0163-8998
    Source: Annual Reviews Electronic Back Volume Collection 1932-2001ff
    Topics: Physics
    Notes: Abstract In the first century of nuclear physics, 31 radioactive elements were added to the periodic system of elements. In 1996, at GSI, element 112 was synthesized by fusion of 70Zn with 208Pb, and its atomic number was established by a decay chain linked to known isotopes. Relativistic mean field calculations of the ground-state stability of nuclei predict the next spherical proton shell not as previously assumed at Z = 114 but at Z = 120 for 304184120. Moreover, a region of spherical nuclei with depleted central density is predicted at N = 172 for 292172120 by mean field calculations. New elements are established today using recoil separators combined with decay-chain analysis. Three new elements, Z = 110-112, and 18 transactinide isotopes have been discovered since 1985, all assigned by genetical linkage to known isotopes. The production cross sections decrease exponentially going to higher elements and now have reached the 1-pb limit. Fusion aiming at higher and higher atomic numbers is a self-terminated process because of constantly increasing disruptive Coulomb forces. The limitations in the formation and deexcitation stages are presented. The rapid drop to smaller cross sections ("Coulomb falls") is modified by nuclear structure not only in the ground state of the final product (superheavy element) but also in the collision partners and during the amalgamation process (closed shells and clusters). The prospects to produce higher elements and new isotopes by extrapolating the physics learned from reaching Z = 112 are 283114, which might be found in 76Ge/208Pb at a level of 0.1 pb and linked to 259No. At this level, about 30 transactinide isotopes are still in reach. To explain the stabilization of production cross sections in the pb range claimed in 1999 experiments, new physics delaying the descent in the "Coulomb falls" is to appear. For the FLNR experiments claiming Z = 114, no explanation is offered. For the LBL experiment claiming Z = 118, an explanation from new physics is presented. All experiments need confirmation. Verifying the centrally depleted, spherical nuclei around 292172120 would be a victory for nuclear structure physics, much more interesting than the trivial case of another doubly closed shell nucleus.
    Type of Medium: Electronic Resource
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  • 2
    Electronic Resource
    Electronic Resource
    Springer
    The European physical journal 220 (1969), S. 101-129 
    ISSN: 1434-601X
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract Delayed neutron emission for thermal neutron fission of235U is investigated by means of a helium-filled mass separator. At the focus of the separator, the neutron activity is detected in coincidence with theΒ decay preceding the neutron emission. Measurements of the activity build-up give the total delayed neutron yield and the yields for different times after fission. Measurements of the activity decay give the half-life distribution. The mass-dependence of yield and half-life was investigated for the whole fission product mass region. The splitting of the total yield of delayed neutrons between light and heavy fission products has been determined. Based on Keepin's value of the total number of delayed neutrons per fission, a yield of 1.05 and 0.53 neutrons per 100 fissions has been obtained for light and heavy fission products, respectively. The experimentally determined mass- and time-dependences of delayed neutron emission are compared with those calculated from the known precursors. Unidentified neutron activities in the mass regions 85–88 (half-life 1 sec) and 96–100 (half-life 1.5 sec) are discussed. By means of theoretical considerations the yield difference for delayed neutrons between light and heavy fission products is interpreted and the new neutron activity is assigned to the precursors98Y or99Y.
    Type of Medium: Electronic Resource
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  • 3
    Electronic Resource
    Electronic Resource
    Springer
    The European physical journal 7 (2000), S. 23-33 
    ISSN: 1434-601X
    Keywords: PACS: 21.10.Dr Binding energies and masses – 23.60.+e α decay – 25.70.-z Low and intermediate energy heavy-ion reactions – 27.90.+b 220 ≤ A
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract: The sequence of radioactive decays of an unknown isotope produced in a rare fusion reaction to known lighter isotopes is used to identify mass and atomic number of the mother isotope, which has been separated before from the bulk of other reaction products by an in-flight recoil separator. By this technique the elements 107 to 112 were produced by single atom decay-chain analysis. Such a correlation technique reaches its limit by the occurrence of accidental sequences and it collapses beyond a maximum possible correlation time, at which a true event cannot be distinguished anymore from a random event. 48Ca-induced fusion reactions with actinides are discussed. In 1983 at GSI, Darmstadt and LBL, Berkeley, 48Ca/248Cm-experiments (II) were performed, which are compared to recent 48Ca-experiments at FLNR-Dubna (I) irradiating 244Pu, 242Pu, and 238U. In these experiments production of isotopes of superheavy elements 112 and 114 is claimed. Our analysis of accidental sequences in 48Ca-induced reactions is presented, which is at variance with the published analysis from FLNR-Dubna. We find that the maximum correlation time using continuous beams at today existing separation systems is not in the one-hour regime, but in the few-minute regime. The five spontaneous fission events observed in the FLNR experiments are preceded by signals in the (1–16)-minute range. These times are shown to be longer than the maximum possible correlation times. The preceding signals are decoupled from the spontaneous fission signal and carry no information on the spontaneous fission events observed. Moreover, random probabilities of 0.2 to 0.6 for the signals preceding the fission events indicate that the correlations are of random origin. The evidence to have discovered element 114 in the reported experiments is classified “very weak”.
    Type of Medium: Electronic Resource
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