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  • Articles: DFG German National Licenses  (3)
  • 1990-1994  (3)
Source
  • Articles: DFG German National Licenses  (3)
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Years
Year
Keywords
  • 1
    Electronic Resource
    Electronic Resource
    Pulse studies of CH4 interaction with NiO/Al2O3 catalysts (1994)
    Springer
    Catalysis letters 27 (1994), S. 199-206 
    Details
    ISSN: 1572-879X
    Keywords: pulse reaction ; NiO/Al2O3 catalysts ; methane activation
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology
    Notes: Abstract Pulse studies of the interaction of CH4 and NiO/Al2O3 catalysts at 500°C indicate that CH4 adsorption on reduced nickel sites is a key step for CH4 oxidative conversion. On an oxygen-rich surface, CH4 conversion is low and the selectivity of CO2 is higher than that of CO. With the consumption of surface oxygen, CO selectivity increases while the CO2 selectivity falls. The conversion of CH4 is small at 500°C when a pulse of CH4/O2 (CH4∶O2=2∶1) is introduced to the partially reduced catalyst, indicating that CH4 and O2 adsorption are competitive steps and the adsorption of O2 is more favorable than CH4 adsorption
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00806993
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    Paper (German National Licenses)
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  • 2
    Electronic Resource
    Electronic Resource
    Oxidative coupling of methane over LaF3/La2O3 catalysts (1994)
    Springer
    Catalysis letters 23 (1994), S. 377-386 
    Details
    ISSN: 1572-879X
    Keywords: Oxidative coupling of methane ; LaF3 ; La2O3 ; rhombohedral LaOF
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology
    Notes: Abstract We studied the oxidative coupling of methane over the LaF3/La2O3 (50∶50) catalyst. The catalyst was found active even at 873 K. At 1023 K, the C2 yield was 12.7% at 26.0% CH4 conversion and 49.1% C2 selectivity. It was found to be stable and had a lifetime not less than 50 h at 1023 K. The catalyst was effective in C2H6 conversion to C2H4. XRD results indicated that the catalyst was mainly rhombohedral LaOF. It is suggested that the catalyst has ample stoichiometric defects and generates active oxygen sites suitable for methane dehydrogenation.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00811372
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    Paper (German National Licenses)
    Fulltext
  • 3
    Electronic Resource
    Electronic Resource
    Exact two-soliton solutions to the Einstein gravitational field equations (1991)
    Springer
    Astrophysics and space science 184 (1991), S. 313-330 
    Details
    ISSN: 1572-946X
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract Following our previous work on the existence of 1-soliton solution to the Einstein gravitational field equations in the presence of a spherically-symmetric static background field, we have found six sets of analytical 2-soliton solutions to the Einstein field equations under a certain ansatz in the absence of the stated background field. Numerical analysis shows that if the two solitons of the transverse nature are injected at space variable z→±∞, the longitudinal field componentg 33 will acquire non-zero values for a bounded spatial region at later time. The nature of the solitons becomes rather complex when they interact. The amplitudeg μν of each soliton may change its magnitude resulting from the interaction. We have found that we might interpret the evolution of one field component as the gravitational instanton in our solutions. We must remark also that the total energy of the interacting solitons remains constant, as expected, at all time. These solutions correspond to the situation where the Riemann tensor is in general non-zero and are truly non-trivial solutions.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00642979
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    Paper (German National Licenses)
    Fulltext
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