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  • 36.40  (2)
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  • 1
    Electronic Resource
    Electronic Resource
    Physical and chemical probes of metallic clusters (1993)
    Springer
    The European physical journal 26 (1993), S. 1-7 
    Details
    ISSN: 1434-6079
    Keywords: 36.40
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract Two different approaches for studying the electronic structure of clusters are presented. The physical probe uses the photoexcitation of size selected alkali-atom clusters. Giant resonances govern the absorption cross-section. It is due to the collective excitation of delocalized valence electrons. The behavior of the resonance up to large sizes, 900-atom clusters for potassium and 1500-atom clusters for lithium puts into evidence the failure of the jellium model for lithium. The chemical approach makes use of the nucleation process in the presence of oxygen. From the analysis of mass spectra of oxidized products, informations are gained on the valence of metallic atom in the cluster oxide. The method is applied to europium and thulium clusters. A comparison is done with the simple case of alkali clusters.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01429095
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    Paper (German National Licenses)
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  • 2
    Electronic Resource
    Electronic Resource
    Stability of alkali-atom clusters (1989)
    Springer
    The European physical journal 12 (1989), S. 199-203 
    Details
    ISSN: 1434-6079
    Keywords: 36.40
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract A detailed study of the stability of alkali-atom clusters is presented and discussed. Free clusters are produced in an unseeded adiabatic expansion and ionized by a pulsed laser beam. A tandem time-of-flight system provides a size selection of ionized species and mass spectrometry of fragments. We have investigated for sodium and potassium clusters containing up to fifty atoms: the metastable decay following ionization, the photo-induced dissociation, the collisional induced dissociation and the collisional charge exchange. Experimental evidence is shown for dissociative process involving evaporation of monomers and dimers. This is explained by the statistical unimolecular theory and by the energetics of the systems.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01426937
    Library Location Call Number Volume/Issue/Year Availability
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    Paper (German National Licenses)
    Fulltext
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