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The solvation of iodine anions in water clusters: PES studies (1993)

Markovich, Gil ; Pollack, Stuart ; Giniger, Rina ; [weitere]

Springer

The European physical journal 26 (1993), S. 98-100

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Details

ISSN: 1434-6079

Schlagwort(e): 36.40.+d ; 33.60.Cv

Quelle: Springer Online Journal Archives 1860-2000

Thema: Physik

Notizen: Abstract We have measured the photoelectron-spectra of I− (H2O)n clusters in the size range n=1–60. We have found that the first six water molecules form a solvation layer with an average 0.35 eV electrostatic stabilization of the anion. At larger cluster sizes the electrostatic stabilization of water does not fit a continuous dielectric solvent. The most stable structures of the clusters consist of internally solvated anions. In the size range n=34–40 we have found evidence for existence of cluster structures with surface solvated anions.

Materialart: Digitale Medien

URL: http://dx.doi.org/10.1007/BF01429115

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