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  • 1
    ISSN: 1432-0630
    Keywords: 61.70 ; 78.70
    Source: Springer Online Journal Archives 1860-2000
    Topics: Mechanical Engineering, Materials Science, Production Engineering, Mining and Metallurgy, Traffic Engineering, Precision Mechanics , Physics
    Notes: Abstract By component analyses of positron lifetime spectra in quenched gold, it was found that positrons are strongly trapped by stacking fault tetrahedra (SFT) at which the lifetime is about 160 ps remarkably smaller than that for monovacancies (∼200 ps) or divacancies (∼220 ps). Positron lifetimes at small vacancy clusters were also estimated in relation to the nucleation process of SFT, with the aid of computer simulation of kinetics of vacancy clustering during quenching and on subsequent isochronal annealing. The results show that large atomic relaxation occurs in small vacancy clusters among which pentavacancies have the largest open-space, thereby having the lifetime of about 230 ps larger than that of trior tetra-vacancies (∼160ps). It is also suggested that tetra- and penta-vacancies act as prenuclei for stable nuclei of SFT consisting of six or more vacancies.
    Type of Medium: Electronic Resource
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  • 2
    Electronic Resource
    Electronic Resource
    Springer
    The European physical journal 26 (1993), S. 180-182 
    ISSN: 1434-6079
    Keywords: 36.40.+d ; 33.80.Eh
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract Electronically excited states of magnesium-water cluster ions, Mg+(H2O) n ,n=1–5, are studied by photodissociation after mass selection. The observed photodissociation spectra are assigned to the2P–2S type transitions localized on the Mg+ ion with the aid of ab initio CI calculations. In addition to evaporation of water molecules, photoinduced intracluster reaction to produce MgOH+(H2O) n is found to occur efficiently, with pronounced size dependence. The intriguing features observed in the mass spectrum of nascent cluster ions are discussed in relation to the stepwise solvation of this reaction.
    Type of Medium: Electronic Resource
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