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  • 1
    Electronic Resource
    Electronic Resource
    Exact solution of a deterministic model for isomerization kinetics (1983)
    Springer
    Journal of statistical physics 33 (1983), S. 317-339 
    Details
    ISSN: 1572-9613
    Keywords: Chemical kinetics ; master equation ; ideal gas ; molecular dynamics ; irreversibility
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract Isomerization kinetics is studied on a one-dimensional ideal gas model with deterministic transitions. The concentrations of species are found to satisfy the phenomenological rate laws appropriate for diffusion-controlled kinetics, and the various correlations are determined. In the long-time regime, higher correlations present long tails reflecting a strongly non-Markovian evolution.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01009800
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