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Effects of freezing out protein vibrational modes on electron transfer kinetics in bacterial reaction centers (1989)

Kakitani, T. ; Mataga, N.

Springer

Photosynthesis research 22 (1989), S. 187-193

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ISSN: 1573-5079

Keywords: electron transfer ; energy gap law ; temperature dependence ; freezing effect ; protein media ; bound water molecules

Source: Springer Online Journal Archives 1860-2000

Topics: Biology

Notes: Abstract We propose a model that some vibrational modes of the protein in bacterial photosynthetic reaction centers may be frozen at low temperatures. The freezing of the protein-environmental motion can affect the electron transfer rate through changes in the reorganization energy and the free energy gap. We offer a qualitative explanation of the different kinetics of the ET processes in reaction centers which are cooled in the dark and cooled under illumination.

Type of Medium: Electronic Resource

URL: http://dx.doi.org/10.1007/BF00048297

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