Abstract
A convenient technique for the ultrashort-relaxation-time measurement using temporally incoherent light instead of short pulses can be applied to the studies of relaxation processes. Theoretical studies on measuring various types of relaxation times by this method are summarized. We have applied this technique to the studies of the electronic dephasing in a polydiacetylene film, the vibrational dephasing in dimethylsulfoxide and the relaxation of optical Kerr effect in CS2 and nitrobenzene.
Similar content being viewed by others
References
H.W. Mocker, R.J. Collins: Appl. Phys. Lett.7, 270 (1965)
C.H. Brito-Cruz, R.L. Fork, C.V. Shank: Opt. Lett.12, 483 (1987)
N. Morita, T. Yajima: Phys. Rev. A30, 2525 (1984)
S. Asaka, H. Nakatsuka, M. Fujiwara, M. Matsuoka: Phys. Rev. A29, 2286 (1984)
R. Beach, S.R. Hartmann: Phys. Rev. Lett.53, 663 (1984)
H. Nakatsuka, M. Tomita, M. Fujiwara, S. Asaka: Opt. Commun.52, 150 (1984)
M. Fujiwara, R. Kuroda, H. Nakatsuka: J. Opt. Soc. Am. B2, 1634 (1985)
S.R. Meech, A.J. Hoff, D.A. Wiersma: Chem. Phys. Lett.121, 287 (1985)
T. Hattori, T. Kobayashi: Chem. Phys. Lett.133, 230 (1987)
A.M. Weiner, S. De Silvestri, E.P. Ippen: J. Opt. Soc. Am. B2, 654 (1985)
A. Laubereau, W. Kaiser: Rev. Mod. Phys.50, 607 (1978)
S.M. George, H. Auwester, C.B. Harris: J. Chem. Phys.73, 5573 (1980)
S.M. George, A.L. Harris, M. Berg, C.B. Harris: J. Chem. Phys.80, 83 (1984)
T. Hattori, A. Terasaki, T. Kobayashi: Phys. Rev. A35, 715 (1987)
M. Tomita, M. Matsuoka: J. Opt. Soc. Am. B3, 560, (1986)
N. Morita, T. Tokizaki, T. Yajima: J. Opt. Soc. Am. B4, 1269 (1987)
K. Kurokawa, T. Hattori, T. Kobayashi: Phys. Rev. A36, 1298 (1987)
N. Morita, K. Torizuka, T. Yajima: J. Opt. Soc. Am. B3, 548 (1986)
E. Wolf: Proc. Phys. Soc. (London)71, 257 (1958)
L. Mandel: Proc. Phys. Soc. (London)74, 223 (1959)
T. Yajima, N. Morita: InMethods of Laser Spectroscopy, ed. by Y. Prior (Plenum, New York 1986), p. 75
R. Beach, D. DeBeer, S.R. Hartmann: Phys. Rev. A32, 3467 (1985)
S.R. Hartmann: IEEE J. QE4, 802 (1968)
R.F. Loring, S. Mukamel: J. Chem. Phys.83, 2116 (1985)
A.C. Eckbreth: Appl. Phys. Lett.32, 421 (1978)
W. Zinth, H.-J. Polland, A. Laubereau, W. Kaiser: Appl. Phys. B26, 77 (1981)
S.M. George, C.B. Harris: Phys. Rev. A28, 863 (1983)
P. Hu, S. Geschwind, T.M. Jedju: Phys. Rev. Lett.37, 1357 (1976)
K.P. Leung, T.W. Mossberg, S.R. Hartmann: Phys. Rev. A25, 3097 (1982)
V. Brückner, E.A.J.M. Bente, J. Langelaar, D. Bebelaar, J.D.W. van Voorst: Opt. Commun.51, 49 (1984)
J.D.W. van Voorst, D. Brandt, B.L. van Hensbergen: In Technical Digest, Topical Meeting on Ultrafast Phenomena (1986)
J.L. Oudar: IEEE J. QE19, 713 (1983)
R.W. Hellwarth: Prog. Quant. Electron.5, 1 (1977)
The possibility of the application of Kerr shutter using incoherent light to luminescence measurement was mentioned first by H. Nakatsuka, ISSP Symposium (December 1987)
S. Koshihara, T. Kobayashi, H. Uchiki, T. Kotaka, H. Ohnuma: Chem. Phys. Lett.114, 446 (1985)
G.M. Carter: J. Opt. Soc. Am. B4, 1018 (1987)
B.I. Greene, J. Orenstein, P.R. Millard, L.R. Williams: Chem. Phys. Lett.139, 381 (1987)
P.P. Ho, N.L. Yang, T. Jimbo, Q.Z. Wang, R.R. Alfano: J. Opt. Soc. Am. B4, 1025 (1987)
T. Kobayashi, J. Iwai, M. Yoshizawa: Chem. Phys. Lett.112, 360 (1984)
T. Kobayashi, H. Ikeda, S. Tsuneyuki: Chem. Phys. Lett.116, 515 (1985)
J. Orenstein, S. Etemad, G.L. Baker: J. Phys. C17, L297 (1984)
L. Robins, J. Orenstein, R. Superfine: Phys. Rev. Lett.56, 1850 (1986)
W.M. Dennis, W. Blau, D.J. Bradley: Appl. Phys. Lett.47, 200 (1985)
G.M. Carter, M.K. Thakur, Y.J. Chen, J.V. Hryniewicz: Appl. Phys. Lett.47, 457 (1985)
D.N. Rao, P. Chopra, S.K. Ghoshal, J. Swiatkiewicz, P.N. Prasad: J. Chem. Phys.84, 7049 (1986)
R.Y. Chiao, E. Garmire, C.H. Townes: Phys. Rev. Lett.13, 479 (1964)
E.P. Ippen, C.V. Shank: Appl. Phys. Lett.26, 92 (1975)
J.M. Halbout, C.L. Tang: Appl. Phys. Lett.40, 765 (1982)
C.L. Tang, J.M. Halbout: InPicosecond Phenomena III, ed. by K.B. Eisenthal, R.W. Hochstrasser, W. Kaiser, A. Laubereau, Springer Ser. Chem. Phys.23 (Springer, Berlin, Heidelberg 1982) p. 212
B.I. Greene, R.C. Farrow: J. Chem. Phys.77, 4779 (1982)
B.I. Greene, R.C. Farrow: InPicosecond Phenomena III, ed. by K.B. Eisentahl, R.W. Hochstrasser, W. Kaiser, A. Laubereau, Springer Ser. Chem. Phys.23 (Springer, Berlin, Heidelberg 1982) p. 209
J. Etchepare, G. Grillon, R. Astier, J.L. Martin, C. Bruneau, A. Antonetti: InPicosecond Phenomena III, ed. by K.B. Eisenthal, R.W. Hochstrasser, W. Kaiser, A. Laubereau, Springer Ser. Chem. Phys.23 (Springer, Berlin, Heidelberg 1982) p. 217
J. Etchepare, G. Grillon, A. Antonetti: Chem. Phys. Lett.107, 489 (1984)
R. Trebino, C.E. Barker, A.E. Siegman: IEEE J. QE,22, 1413 (1986)
C. Kalpouzos, W.T. Lotshaw, D. McMorrow, G.A. Kenney-Wallace: J. Phys. Chem.91, 2028 (1987)
S. Ruhman, L.R. Williams, A.G. Joly, B. Kohler, K.A. Nelson: J. Phys. Chem.91, 2237 (1987)
J. Etchepare, G. Grillon, J.P. Chambaret, G. Hamoniaux, A. Orszag: Opt. Commun.63, 329 (1987)
M. Golombok, G.A. Kenney-Wallace: InUltrafast Phenomena IV, ed. by D.H. Auston, K.B. Eisenthal, Springer Ser. Chem. Phys.38 (Springer, Berlin, Heidelberg 1987) p. 383
J. Etchepare, G. Grillon, I. Thomazeau, A. Migus, A. Antonetti: J. Opt. Soc. Am B2, 649 (1985)
Author information
Authors and Affiliations
Rights and permissions
About this article
Cite this article
Kobayashi, T., Terasaki, A., Hattori, T. et al. The application of incoherent light for the study of femtosecond-picosecond relaxation in condensed phase. Appl. Phys. B 47, 107–125 (1988). https://doi.org/10.1007/BF00684078
Received:
Accepted:
Issue Date:
DOI: https://doi.org/10.1007/BF00684078