Conclusions
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1.
The generation of radiation in a complex system consisting of a material with intense SpRS lines and generating-dye molecules, situated in a common resonator due to connectedness over the field, occurs at the peak amplification frequencies of the system as a whole.
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2.
With a favorable disposition of the scattered-light lines and amplification and generation band of a dye solution, the emission spectrum of a composite system contains systems of SpRS lines of the substance, which do not as a rule appear in the StRS spectrum.
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3.
A purpose-designed system makes it possible to obtain an active medium with a lower generation threshold than those exhibited by its individual components; such a system gives a narrow (narrower than 1 cm−1) generation line.
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Additional information
Translated from Zhurnal Prikladnoi Spektroskopii, Vol. 9, No. 5, pp. 784–788, November, 1968.
We are grateful to G. G. Dyadyusha for several useful remarks in connection with this paper.
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Tikhonov, E.A., Shpak, M.T. Light generation by systems of liquid solutions of organic dyes with negative absorption at the activator molecules and induced Raman scattering at the matrix molecules. J Appl Spectrosc 9, 1197–1200 (1968). https://doi.org/10.1007/BF00696400
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DOI: https://doi.org/10.1007/BF00696400