Abstract
Measurements at Barrow during the second Arctic Gas and Aerosol Sampling Program (AGASP-II), conducted in April 1986, showed no rapid long-range transport from lower-latitude source regions to Barrow, and only limited vertical transport from above the boundary layer to the surface. New aerosol size distribution measurements in the 0.005–0.1 μm diameter size range using a Nuclepore-filter diffusion battery apparatus showed a median diameter of about 0.01 μm during times of high condensation nucleus (CN) concentrations. Aerosol black carbon concentrations exceeding 400 ng m−3 were detected at the surface and were more strongly correlated with CN concentrations than with aerosol scattering extinction (σsp), suggesting that aerosol carbon was generally associated with small particles rather than large particles. Measurements at Barrow during AGASP-I, conducted in March–April 1983, showed a series of aerosol events detected at the ground that were caused by rapid long-range transport paths to the vicinity of Barrow from Eurasia. These events were strongly correlated with aerosol loading in the vertical column (optical depth).
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References
Ahlquist, N. C., and R. J. Charlson, 1969, “Measurement of the wavelength dependence of atmospheric extinction due to scatter” Atmos. Environ. 3, 551–564.
Allen, M. D., and Raabe, O. G., 1982, “Re-evaluation of Millikan's oil drop data for the motion of small particles in air,” Aerosol Sci. 13, 537–547.
Bodhaine, B. A., 1979, “Measurement of the Rayleigh scattering properties of some gases with a nephelometer,” Appl. Opt. 18, 121–125.
Bodhaine, B. A., 1983, “Aerosol measurements at four background sites,” J. Geophys. Res. 88, 10753–10768.
Bodhaine, B. A., and J. J. DeLuisi, 1985, “An aerosol climatology of Samoa,” J. Atmos. Chem. 3, 107–122.
Bodhaine, B. A., and M. E. Murphy, 1980, “Calibration of an automatic condensation nuclei counter at the South Pole,” J. Aerosol Sci. 11, 305–312.
Bodhaine, B. A., J. M. Harris, and G. A. Herbert, 1981, “Aerosol light scattering and condensation nuclei measurements at Barrow, Alaska,” Atmos. Environ. 15, 1375–1389.
Bodhaine, B. A., E. G. Dutton, and J. J. DeLuisi, 1984, “Surface aerosol measurements at Barrow during AGASP,” Geophys. Res. Lett. 11, 377–380.
Dutton, E. G., J. J. DeLuisi, and B. A. Bodhaine, 1984, “Features of aerosol optical depth observed at Barrow, March 10–20, 1983,” Geophys. Res. Lett. 11, 385–388.
Hansen, A. D. A., H. Rosen, and T. Novakov, 1982, “Real-time measurement of the absorption coefficient of aerosol particles,” Appl. Opt. 21, 3060–3062.
Harris, J. M., 1984, “Trajectories during AGASP,” Geophys. Res. Lett. 11, 453–456.
Heidam, N. Z., 1981, “Review: Aerosol fractionation by sequential filtration with Nuclepore filters,” Atmos. Environ. 15, 891–904.
Herbert, G. A., H. A. Bridgman, R. C. Schnell, B. A. Bodhaine, and S. J. Oltmans, 1989, “Meteorology and haze structure during AGASP II: Alaskan Arctic flights, April 2–10, 1986,” J. Atmos. Chem., this issue.
Komhyr, W. D., 1983, “An aerosol and gas sampling apparatus for remote observatory use,” J. Geophys. Res. 88, 3913–3918.
Metnieks, A. L., and L. W. Pollak, 1959, “Instruction for use of photo-electric condensation nucleus counters,” Geophys. Bull. 16, School of Cosmic Physics, Dublin Institute for Advanced Study, Dublin, Ireland.
Miller, S. W., and B. A. Bodhaine, 1982, “Supersaturation and expansion ratios in condensation nuclei counters: An historical perspective,” J. Aerosol Sci. 13, 481–490.
Murphy, M. E., and B. A. Bodhaine, 1980, “The Barrow, Alaska automatic condensation nuclei counter and four wavelength nephelometer: Instrument details and four years of observations,” NOAA Tech. Memo. ERL ARL-90, Air Resources Laboratory, Silver Spring, MD, 101 pp.
Quakenbush, T. K., and B. A. Bodhaine, 1986, “Surface aerosols at the Barrow GMCC observatory: Data from 1976 through 1985,” NOAA Data Rep. ERL ARL-10, Air Resources Laboratory, Silver Springer, MD, 230 pp.
Raatz, W. E., 1984, “Tropospheric circulation patterns during the Arctic Gas and Aerosol Sampling Program (AGASP), March/April 1983,” Geophys. Res. Lett. 11, 449–452.
Raatz, W. E., R. C. Schnell, B. A. Bodhaine, S. J. Oltmans, and R. H. Gammon, 1985, “Air mass characteristics in the vicinity of Barrow, Alaska, 9–19 March 1983,” Atmos. Environ. 19, 2127–2134.
Rosen, H., A. D. A. Hansen, L. Gundel, and T. Novakov, 1978, “Identification of the optically absorbing component in urban aerosols,” Appl. Opt. 17, 3859–3861.
Schnell, R. C., 1984, “Arctic haze and the Arctic Gas and Aerosol Sampling Program (AGASP),” Geophys. Res. Lett. 11, 361–364
Schnell, R. C., T. Watson, and B. A. Bodhaine, 1989, “NOAA WP-3D instrumentation and flight operations on AGASP-II,” J. Atmos. Chem., this issue.
Shaw, G. E., 1985, “On very small particles in the Alaska Arctic troposphere,” J. Rech. Atmos. 19, 235–242.
Skala, G. F., 1963, “A new instrument for the continuous measurement of condensation nuclei,” Anal. Chem. 35, 702–706.
Thielke, J. F., R. J. Charlson, J. W. Winter, N. C. Ahlquist, K. T. Whitby, R. B. Husar, and B. Y. H. Liu, 1972, “Multiwavelength nephelometer measurements in Los Angeles smog aerosols, II. Correlation with size distributions, volume concentrations,” J. Colloid Inter. Sci. 39, 252–259.
Twomey, S., 1975, “Comparison of constrained linear inversion and an iterative nonlinear algorithm applied to the indirect estimation of particle size distributions,” J. Comp. Phys. 18, 188–200.
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Bodhaine, B.A., Dutton, E.G., DeLuisi, J.J. et al. Surface aerosol measurements at Barrow during AGASP-II. J Atmos Chem 9, 213–224 (1989). https://doi.org/10.1007/BF00052833
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DOI: https://doi.org/10.1007/BF00052833