Library

Your email was sent successfully. Check your inbox.

An error occurred while sending the email. Please try again.

Proceed reservation?

Export
Filter
  • Electronic Resource  (3)
  • E-Resource
  • Loose Leaf
  • 2000-2004  (3)
  • 2001  (3)
  • PACS. 31.70.Hq Time-dependent phenomena: excitation and relaxation processes, and reaction rates – 33.80.Wz Other multiphoton processes  (2)
  • AMS Classification. 65L05; 22E60.  (1)
Material
  • Electronic Resource  (3)
  • E-Resource
  • Loose Leaf
Years
  • 2000-2004  (3)
Year
  • 2001  (3)
Keywords
  • 1
    ISSN: 1434-6079
    Keywords: PACS. 31.70.Hq Time-dependent phenomena: excitation and relaxation processes, and reaction rates – 33.80.Wz Other multiphoton processes
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract: We present simulations on pump-dump-probe experiments performed on the potassium dimer. The interaction of two time-delayed laser pulses prepares vibrational wave packets in the electronic ground state. The quantum calculations reveal to what extent it is possible to prepare a ground state superposition of states with high versus low vibrational quantum numbers by changing the pump-dump delay time. It is shown that transient signals may exhibit interference effects which are due to characteristics of ground state wave-packets composed of two components showing different vibrational dynamics. In this way the signals are able to yield information about vibrational overtone motion.
    Type of Medium: Electronic Resource
    Library Location Call Number Volume/Issue/Year Availability
    BibTip Others were also interested in ...
  • 2
    Electronic Resource
    Electronic Resource
    Springer
    Foundations of computational mathematics 1 (2001), S. 129-160 
    ISSN: 1615-3383
    Keywords: AMS Classification. 65L05; 22E60.
    Source: Springer Online Journal Archives 1860-2000
    Topics: Mathematics
    Notes: Abstract. In this paper we develop in a systematic manner the theory of time-stepping methods based on the Cayley transform. Such methods can be applied to discretize differential equations that evolve in some Lie groups, in particular in the orthogonal group and the symplectic group. Unlike many other Lie-group solvers, they do not require the evaluation of matrix exponentials. Similarly to the theory of Magnus expansions in [13], we identify terms in a Cayley expansion with rooted trees, which can be constructed recursively. Each such term is an integral over a polytope but all such integrals can be evaluated to high order by using special quadrature formulas similar to the construction in [13]. Truncated Cayley expansions (with exact integrals) need not be time-symmetric, hence the method does not display the usual advantages associated with time symmetry, e.g., even order of approximation. However, time symmetry (with its attendant benefits) is attained when exact integrals are replaced by certain quadrature formulas.
    Type of Medium: Electronic Resource
    Library Location Call Number Volume/Issue/Year Availability
    BibTip Others were also interested in ...
  • 3
    Electronic Resource
    Electronic Resource
    Springer
    The European physical journal 15 (2001), S. 413-422 
    ISSN: 1434-6079
    Keywords: PACS. 31.70.Hq Time-dependent phenomena: excitation and relaxation processes, and reaction rates – 33.80.Wz Other multiphoton processes
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract: A classical approach to simulate femtosecond pump-probe experiments is presented and compared to the quantum mechanical treatment. We restrict the study to gas-phase systems using the I2 molecule as a numerical example. Thus, no relaxation processes are included. This allows for a direct comparison between purely quantum mechanical results and those obtained from classical trajectory calculations. The classical theory is derived from the phase-space representation of quantum mechanics. Various approximate quantum mechanical treatments are compared to their classical counterparts. Thereby it is demonstrated that the representation of the radial density as prepared in the pump-process is most crucial to obtain reliable signals within the classical approach.
    Type of Medium: Electronic Resource
    Library Location Call Number Volume/Issue/Year Availability
    BibTip Others were also interested in ...
Close ⊗
This website uses cookies and the analysis tool Matomo. More information can be found here...