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Unimolecular activation-deactivation: Impulsive collision theory (1981)

Schranz, Harold W. ; Nordholm, Sture

New York, NY : Wiley-Blackwell

International Journal of Chemical Kinetics 13 (1981), S. 1051-1070

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ISSN: 0538-8066

Keywords: Chemistry ; Physical Chemistry

Source: Wiley InterScience Backfile Collection 1832-2000

Topics: Chemistry and Pharmacology

Notes: A theory of collisional energy transfer based on microcanonical relaxation in the limit of infinitesimal collision lifetimes is developed. In distinction to the recently formulated ergodic collision theory the potential energy is now frozen due to the short time scale, and only kinetic energy is available for redistribution. As a consequence, the rate of energy transfer is decreased, and agreement with experimentally based estimates generally improved.

Additional Material: 1 Ill.

Type of Medium: Electronic Resource

URL: http://dx.doi.org/10.1002/kin.550131006

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