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Superselectivity and solvation forces of a two component fluid adsorbed in slit micropores (1993)

Somers, Susan A. ; McCormick, Alon V. ; Davis, H. Ted

College Park, Md. : American Institute of Physics (AIP)

The Journal of Chemical Physics 99 (1993), S. 9890-9898

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ISSN: 1089-7690

Source: AIP Digital Archive

Topics: Physics , Chemistry and Pharmacology

Notes: We use the grand canonical Monte Carlo simulation technique to calculate adsorption of mixtures in molecularly narrow slit pores immersed in a two-component bath of spherical molecules that are different in size. The composition of the pore fluid oscillates strongly with the pore width. The oscillations reflect the differing ability of each molecule to pack as layers in the pore. Even in pores wide enough to admit both components, this difference in packing ability leads to a shut-out of the smaller component. Trends in the calculated solvation force agree with both experiment and theory.

Type of Medium: Electronic Resource

URL: http://dx.doi.org/10.1063/1.465473

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