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On the hard sphere bridge function (1992)

Taylor, Mark P. ; Lipson, J. E. G.

College Park, Md. : American Institute of Physics (AIP)

The Journal of Chemical Physics 97 (1992), S. 7851-7852

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ISSN: 1089-7690

Source: AIP Digital Archive

Topics: Physics , Chemistry and Pharmacology

Notes: The bridge function for a simple fluid can be written as a diagrammatic expansion involving either the Mayer f-function f(r) or the total correlation function h(r). At each order, the h-bond expansion includes all f-bond diagrams to that order plus an infinite subset of higher order f-bond diagrams. Thus, taken to any order, the h-bond expansion is generally considered more accurate than the f-bond expansion. However, here we show that for hard spheres, the lowest order h-bond approximation for the bridge function is much less accurate than the corresponding f-bond approximation.

Type of Medium: Electronic Resource

URL: http://dx.doi.org/10.1063/1.463459

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