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Dynamics of the oxidation of CO on Pt(111) by an atomic oxygen beam (1991)

Mullins, C. B. ; Rettner, C. T. ; Auerbach, D. J.

College Park, Md. : American Institute of Physics (AIP)

The Journal of Chemical Physics 95 (1991), S. 8649-8651

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ISSN: 1089-7690

Source: AIP Digital Archive

Topics: Physics , Chemistry and Pharmacology

Notes: We have determined the angular and velocity distributions of the CO2 product of the interaction of gas-phase O atoms with CO adsorbed on Pt(111) at 90 K. The desorption intensity is found to be strongly peaked along the surface normal, falling approximately as cos12 θf with increasing final angle, θf. The velocity distributions are found to be highly non-Boltzmann with mean energies of ∼0.6 eV, decreasing slightly with increasing θf.

Type of Medium: Electronic Resource

URL: http://dx.doi.org/10.1063/1.461244

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