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Temperature dependence of the rate of the electronic-to-electronic energy transfer from NF(b 1Σ+) to IF (1986)

Pritt, A. T. ; Benard, D. J.

College Park, Md. : American Institute of Physics (AIP)

The Journal of Chemical Physics 85 (1986), S. 7159-7166

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ISSN: 1089-7690

Source: AIP Digital Archive

Topics: Physics , Chemistry and Pharmacology

Notes: The temperature dependence of the rate of transfer of electronic energy from NF(b 1Σ+) to ground state IF(X 1Σ+) to form IF[B 3Π(O+)] has been determined using a chemiluminescence flowtube apparatus. The energy transfer rate depends on the vibrational distribution of the IF(X 1Σ+), but is independent of the vibrational distribution of the NF(b 1Σ+). The vibrational temperature of the IF[B 3Π(O+)] product was also greater than or equal to the vibrational temperature of the IF(X 1Σ+) reagent. These results are explained in terms of an energy transfer model requiring that the individual state-to-state rates are proportional to the corresponding Franck–Condon factors.

Type of Medium: Electronic Resource

URL: http://dx.doi.org/10.1063/1.451349

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