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Small pore closure and the deactivation of the limestone sulfation reaction (1986)

Simons, G. A. ; Garman, A. R.

Hoboken, NJ : Wiley-Blackwell

AIChE Journal 32 (1986), S. 1491-1499

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ISSN: 0001-1541

Keywords: Chemistry ; Chemical Engineering

Source: Wiley InterScience Backfile Collection 1832-2000

Topics: Chemistry and Pharmacology , Process Engineering, Biotechnology, Nutrition Technology

Notes: The sulfation model of Simons and Rawlins (1980) is extended to include the effect of product deposits. The model includes: 1. the plugging of the smallest pores and the subsequent loss in the internal surface area, 2. the diffusion of the SO2 through the product deposits, and 3. the loss of intraparticle diffusion due to the complete plugging of the largest pores. It is shown that the plugging of the smallest pores is generally rate-controlling.

Additional Material: 10 Ill.

Type of Medium: Electronic Resource

URL: http://dx.doi.org/10.1002/aic.690320910

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