Electronic Resource
College Park, Md.
:
American Institute of Physics (AIP)
The Journal of Chemical Physics
104 (1996), S. 7068-7072
ISSN:
1089-7690
Source:
AIP Digital Archive
Topics:
Physics
,
Chemistry and Pharmacology
Notes:
Highly efficient population transfer between the (0,0,0) and the (9,1,0) vibrational levels of the electronic ground state X˜ 1A1 of SO2 is demonstrated. The process relies on stimulated Raman scattering with adiabatic passage induced by two suitably delayed ultraviolet laser pulses with nearly transform-limited bandwidth. A transfer efficiency of 100% is achieved. The associated dark resonance is observed. Properties of the latter are compared for delayed and fully overlapping pulses. © 1996 American Institute of Physics.
Type of Medium:
Electronic Resource
URL:
http://dx.doi.org/10.1063/1.471424
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