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Catalytic reaction accompanied by capillary condensation, 3. Influence on reaction kinetics and dynamics (1998)

Bukhavtsova, N. M. ; Ostrovskii, N. M.

Springer

Reaction kinetics and catalysis letters 65 (1998), S. 321-329

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ISSN: 1588-2837

Keywords: Catalytic reaction ; capillary condensation ; kinetics ; dynamics

Source: Springer Online Journal Archives 1860-2000

Topics: Chemistry and Pharmacology

Notes: Abstract The influence of capillary condensation of reagents on the catalytic reaction kinetics and dynamics was studied. The hydrogenation ofp-xylene over Pt/SiO2 was used as a model reaction. Two types of SiO2 were used (KCK-1 with large pores and KCM-5 with small pores). It was shown that capillary condensation could modify the kinetics and the transition regimes. The proposed mathematical model demonstrates good agreement with experimental results for both steady-state and dynamic regimes, including reaction rate—temperature hysteresis.

Type of Medium: Electronic Resource

URL: http://dx.doi.org/10.1007/BF02475271

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