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Linear prediction and resolution enhancement of complex line shapes in two-dimensional electron-spin-echo spectroscopy (1986)

Millhauser, G. L. ; Freed, J. H.

College Park, Md. : American Institute of Physics (AIP)

The Journal of Chemical Physics 85 (1986), S. 63-67

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ISSN: 1089-7690

Quelle: AIP Digital Archive

Thema: Physik , Chemie und Pharmazie

Notizen: A new type of two-dimensional electron-spin-echo (2D-ESE) spectroscopy was recently shown to be useful for studying slow molecular motions in liquids. A recently developed method of spectral enhancement based upon linear prediction with singular value decomposition (LPSVD) is applied in the present work to dramatically improve the signal-to-noise ratio and to correct for finite dead time in the data from this 2D-ESE experiment. This permitted a more accurate comparison between theory and experiment. Good agreement is now obtained with a model of nearly isotropic Brownian motion for tempone in glycerol/water solvent.

Materialart: Digitale Medien

URL: http://dx.doi.org/10.1063/1.451595

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