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  • 1
    Electronic Resource
    Electronic Resource
    Woodbury, NY : American Institute of Physics (AIP)
    Applied Physics Letters 64 (1994), S. 3365-3367 
    ISSN: 1077-3118
    Source: AIP Digital Archive
    Topics: Physics
    Notes: We demonstrate intersubband absorption and second harmonic generation (SHG) in asymmetric coupled In0.6Ga0.4As/AlAs n-type quantum wells (QWs) grown on a GaAs substrate. Intersubband absorption at 4.1 and 2.1 μm wavelengths, corresponding to the 1 to 2 and 1 to 3 transitions, respectively, are observed. SHG of 2.0 μm light is demonstrated in this doubly resonant QW. This is the shortest wavelength SHG to date in any n-type QW system. The second order nonlinear susceptibility χ(2) is measured using a free electron laser by interference of the second harmonic fields from the QW and substrate. At a pump wavelength of 4.0 μm, a large asymmetry in the SHG power with rotation angle of the sample arising from SHG from the QW is observed, and a χ(2) of magnitude 20±8 nm/V, approximately 100 times that of bulk GaAs, and phase 63°±34° relative to the GaAs substrate is measured. Comparison of both the linear and nonlinear properties to a simple model is discussed.
    Type of Medium: Electronic Resource
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  • 2
    ISSN: 1077-3118
    Source: AIP Digital Archive
    Topics: Physics
    Notes: We report short wavelength second-harmonic generation (SHG) spectroscopy of asymmetric coupled In0.6Ga0.4As/AlAs quantum wells (QWs). The QW is designed to show maximum second-order nonlinear susceptibility χ(2) for SHG of 4 and 2 μm wavelengths by single and double resonance effects, respectively. SHG spectroscopy across the midinfrared is measured using both a CO2 and a free electron laser as pumps. The χ(2) of the QW is extracted from interference of the second-harmonic fields from the QW and GaAs substrate, determined by the azimuthal dependence of the SHG power. We measure χ(2) of the QW for harmonic wavelengths between 5.36 and 1.85 μm. This is the shortest wavelength SHG to date by any QW intersubband interaction. Good agreement of experiment with theory for the dispersion of χ(2) for both singly and doubly resonant conversion is observed throughout the midinfrared. © 1994 American Institute of Physics.
    Type of Medium: Electronic Resource
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