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  • 1990-1994  (3)
  • 1
    Electronic Resource
    Electronic Resource
    [S.l.] : American Institute of Physics (AIP)
    Journal of Applied Physics 69 (1991), S. 4409-4417 
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: The removal of SO2 from simulated gas streams (N2/O2/H2O/SO2) is experimentally investigated using a dielectric barrier discharge, and by computer modeling. Conversion of SO2 to primarily H2SO4 is found to be limited by the generation of OH radicals. Increasing the concentrations of O2 and H2O increases the generation of OH radicals and results in more removal of SO2 from gas streams. Removal efficiencies of (approximately-greater-than)80% were experimentally achieved. Results from the model suggest that more efficient removal is obtained with a series of short, high E/N current pulses rather than a single, low E/N current pulse. Results from the model also suggest that uv illumination of the plasma to photolyze O3 will improve the removal of SO2 from the gas stream. Photolysis of O3 produces O(1D) atoms which generate OH radicals by H abstraction from H2O, thereby increasing the removal of SO2.
    Type of Medium: Electronic Resource
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  • 2
    Electronic Resource
    Electronic Resource
    s.l. : American Chemical Society
    Environmental science & technology 26 (1992), S. 777-781 
    ISSN: 1520-5851
    Source: ACS Legacy Archives
    Topics: Chemistry and Pharmacology , Energy, Environment Protection, Nuclear Power Engineering
    Type of Medium: Electronic Resource
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  • 3
    ISSN: 1572-8986
    Keywords: Dielectric barrier discharge ; SO2 removal ; NO removal ; gasphase oxidation
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology , Mechanical Engineering, Materials Science, Production Engineering, Mining and Metallurgy, Traffic Engineering, Precision Mechanics , Technology
    Notes: Abstract A gas-phase oxidation method using dielectric barrier discharges (DBDs) has been developed to remove SO2 and to simultaneously remove SO2 and NO from gas streams that are similar to gas streams generated by the combustion of fossil fuels. SO2 and NO removal efficiencies are evaluated as a function of applied voltage, temperature, and concentrations of SO2, NO, H2O(g), and NH3. With constant H2O(g) concentration, both SO2 and NO removal efficiencies increase with increasing temperature from 100 to 160°C. At 160°C with 15% by volume H20(g), more than 95% of the NO and 32% of the S02 are simultaneously removed from the gas stream. Injection of NH3 into the gas stream caused an increase in S02 removal efficiency to essentially 100%. These results indicate that DBD plasmas have the potential to simultaneously remove SO2 and NO from gas streams generated by large-scale fossil fuel combustors.
    Type of Medium: Electronic Resource
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