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  • Articles: DFG German National Licenses  (26)
  • Chemistry  (23)
  • 21.60.−n  (3)
  • 1
    Electronic Resource
    Electronic Resource
    The115In(γ, γ′) reaction as a test of the quasi-particle phonon model with complex configurations in odd-mass nuclei (1995)
    Springer
    The European physical journal 350 (1995), S. 303-309 
    Details
    ISSN: 1434-601X
    Keywords: 21.10.Tg ; 21.60.−n ; 25.20.Lj ; 27.60.+j
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract The115In(γ, γ′) reaction was measured at the S-DALINAC using bremsstrahlung with endpoint energiesE 0=3.1, 4.6 and 5.2 MeV. In the excitation energy range of 1–5 MeV in total 32 transitions were observed, 18 of which were hithertoo unknown. The results are compared to two quasiparticle-phonon model calculations, one with a model space of ‘quasiparticle⊗phonon’ and one extended by ‘quasiparticle⊗two-phonon’ configurations. A substantial improvement is achieved in the description of low-lying115In states by the consideration of the more complex configurations. The calculations quantitatively account for the summed115In(γ, γ′) integrated cross sections and show a comparable amount of fragmentation of the individual transition strengths. The model interpretation of the microscopic structure of the experimentally observed transitions is discussed.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01291187
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  • 2
    Electronic Resource
    Electronic Resource
    Super-allowed beta decay of nuclei at the drip-line (1991)
    Springer
    The European physical journal 340 (1991), S. 255-261 
    Details
    ISSN: 1434-601X
    Keywords: 23.40.Hc ; 21.60.−n ; 27.20.+n
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract We have investigated the continuous particle spectra following the beta decay of the neutron-rich nuclei that terminate the mass 6, 8, 9 and 11 isobaric chains. Strong beta transitions feeding the very top of the spectrum are found systematically. The favoured states are within a few MeV of the energy of the initial state. This phenomenon seems to be linked to the occurrence of a di-neutron structure or neutron halo in the drip-line nuclei.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01294673
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  • 3
    Electronic Resource
    Electronic Resource
    Phenomenological wave functions for the massA=14 system and a consistent description of beta decay observables (1991)
    Springer
    The European physical journal 341 (1991), S. 9-24 
    Details
    ISSN: 1434-601X
    Keywords: 21.60.−n ; 23.40.−s ; 25.30.−c
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract A set of phenomenological wave functions has been derived to describe the14N ground state and the isospin triplet consisting of the14C ground state, the first excited state of14N at 2.313 MeV and the14O ground state. Elastic and inelastic electron scattering form factors, the magnetic moment of the14N ground state and the shape factors in theβ ± decay have been employed in a multiparameter fitting procedure to determine the amplitudes of the wave functions inL-S coupling. The inclusion of the beta decay observables in the fit has become possible for the first time since exact formulas for the shape factor in higher order do exist. The set of wave functions deduced exhibit predominately anL=0 contribution for the 0+; 1 states andL=1 and 2 contributions of nearly equal weight for the 1+; 0 state. It was observed that the inclusion of the shape factors allowed a more stringent determination of the amplitudes compared to previous attempts reported in the literature and led in the case of the 0+; 1 states to wave functions that show a small but noticeable difference within the isospin triplet. Besides the observables used for the fit, the radiative widthΓ γ (M1) of the 2.313 MeV state in14N can be described quite well with the derived wave functions, and in addition it has become possible to predict the pathological largeft − value of the14C decay and theft + value of the14O decay precisely. The wave functions are also applied to calculate the14N(γ,π +) cross section.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01281270
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  • 4
    Electronic Resource
    Electronic Resource
    Arylierung von Thiocarbonylverbindungen mit Diazoniumsalzen (1982)
    New York, NY : Wiley-Blackwell
    Journal für Praktische Chemie/Chemiker-Zeitung 324 (1982), S. 669-672 
    Details
    ISSN: 0021-8383
    Keywords: Chemistry ; Organic Chemistry
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Chemistry and Pharmacology
    Notes: Arylation of Thiocarbonyl Compounds by Arenediazonium Salts
    Additional Material: 1 Tab.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1002/prac.19823240425
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  • 5
    Electronic Resource
    Electronic Resource
    Synthese und Oxydation von 1-(1,3-Thiazol-2-yl)-pyrazolid-3-onen (1982)
    New York, NY : Wiley-Blackwell
    Journal für Praktische Chemie/Chemiker-Zeitung 324 (1982), S. 873-881 
    Details
    ISSN: 0021-8383
    Keywords: Chemistry ; Organic Chemistry
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Chemistry and Pharmacology
    Notes: Synthesis and Oxydation of 1-(1,3-Thiazol-2-yl)-pyrazolidin-3-onesThe 1-(1,3-thiazol-2-yl)-pyrazolid-3-ones 4 are synthesized by reaction of 1-thiocarbamoyl-pyrazolidin-3-one 2 with α-halogenaldehydes and α-halogenketones, respectively. The structure of 4 is proved by their 1H-n.m.r. and mass spectra. Oxydative dimerisation of 4 leads to the bisazomethinimines 10. The compounds 10 represent a new type of azomethinimines with a quinoid structure.
    Additional Material: 1 Ill.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1002/prac.19823240602
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  • 6
    Electronic Resource
    Electronic Resource
    Tetrathiafulvalene. XXI. Synthese von Tetrathiafulvalenen aus 2-Alkylthio-, 2-Arylthio- und 2-Alkylseleno-1,3-dithioliumsalzen (1984)
    New York, NY : Wiley-Blackwell
    Journal für Praktische Chemie/Chemiker-Zeitung 326 (1984), S. 479-484 
    Details
    ISSN: 0021-8383
    Keywords: Chemistry ; Organic Chemistry
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Chemistry and Pharmacology
    Notes: Tetrathiafulvalenes. XXI. Syntheses of Tetrathiafulvalenes from 2-Alkylthio-, 2-Arylthio- and 2-Alkylseleno-1,3-dithiolium SaltsIn the reaction of 2-alkylthio-, 2-arylthio- or 2-alkylseleno-1, 3-dithiolium salts with trivalent phosphorus compounds in acetonitril tetrathiafulvalenes 2 are formed. As an intermediate we suppose a phosphorane, which reacts with further 1,3-dithiolium salt to provide the tetrathiafulvalene. By the application of a 2-alkylthio-1,3-dithiolium salt a monomethin dye is formed in a side reaction. When the reaction is carried out in methanol, the phosphorane is trapped by the solvent and a 2H-1,3-dithiolium salt is obtained.
    Additional Material: 2 Tab.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1002/prac.19843260316
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  • 7
    Electronic Resource
    Electronic Resource
    Zur Chlorierung von N-Aryl-2,4-dimethyl-buta-1,3-dien-1,4-sultamenHerrn Prof. Dr. J. Ulbricht zum 60. Geburtstag gewidmet (1984)
    New York, NY : Wiley-Blackwell
    Journal für Praktische Chemie/Chemiker-Zeitung 326 (1984), S. 545-555 
    Details
    ISSN: 0021-8383
    Keywords: Chemistry ; Organic Chemistry
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Chemistry and Pharmacology
    Notes: About Chlorination of N-Aryl-2,4-dimethyl-buta-1,3-dien-1,4-sultamesThe sultames of structure 1 are easily chlorinated by sulfurylchloride, chlorine or tertbutylhypochlorite. The structure of the mono-(2a-c,3a, d), di-(4a-d), tri- (5c, d) and pentachlorosultames (6a, b) is determined by 13C-n.m.r. spectroscopy. Contrary to the bromination the chlorination (by SO2Cl2) starts with the substitution of the sultamring (formation of mono- and di-chlorosultames) followed of the substitution of the (C-4)-CH3- group (formation of trichlorosultames). By 1,4-addition of an other molecule of chlorine to 5 the pentachlorosultames 6a, b are obtained. Already by recrystalisation of 6a, b in an alcohol the chlorine in 4-position is exchanged by the corresponding alkoxy group (CH3O, C2H5O, n-C3H7O) and the compounds 7-9 are formed.
    Additional Material: 5 Tab.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1002/prac.19843260404
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  • 8
    Electronic Resource
    Electronic Resource
    Organische Elektronenleiter und Vorstufen. V.IV. Mitt.: RICHTER, A. M.; FANGHÄNEL E.: Sulfur Lett. 3 (1985) 25. Synthese von Poly(organylthio-acetylenen) (1987)
    New York, NY : Wiley-Blackwell
    Journal für Praktische Chemie/Chemiker-Zeitung 329 (1987), S. 811-816 
    Details
    ISSN: 0021-8383
    Keywords: Chemistry ; Organic Chemistry
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Chemistry and Pharmacology
    Notes: Organic Electron Conductors and Precursors. V. Synthesis of Poly (organylthio-acetylenes)Poly(bis-organylthio-acetylenes) 2 and poly(mono-organylthio-acetylenes) 3 have been synthesized by complex catalyzed polymerization of the corresponding acetylenes (4 resp. 5). Yields and properties of the polymers 2, 3 depend on reaction conditions, the catalyst and the nature of the acetylenes. Relations between these influence factors are discussed.
    Additional Material: 3 Tab.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1002/prac.19873290509
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  • 9
    Electronic Resource
    Electronic Resource
    Iodierung von N-Aryl-2,4-dimethyl-buta-1,3-dien-1,4-sultamen (1985)
    New York, NY : Wiley-Blackwell
    Journal für Praktische Chemie/Chemiker-Zeitung 327 (1985), S. 428-432 
    Details
    ISSN: 0021-8383
    Keywords: Chemistry ; Organic Chemistry
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Chemistry and Pharmacology
    Notes: Iodation of N-Aryl-2,4-dimethyl-buta-1,3-dien-1,4-sultamesBy the iodation of N-aryl-2,4-dimethyl-buta-1,3-dien-1,4-sultames 1 with I2/HgO in EtOH/AcOH the 1,2-thiazine ring is substituted. The monosubstitution occurs on the 1-position (1a, d) and the disubstitution on the 1,3-position (3a). By iodine monochloride in CHCl3 the sultames 1a-d were substituted in the (C-2)-CH3 group (4a-d), in contrast also to the results of chlorination and bromination of 1. The structure of the products 2, 3, 4 was proved by 13C-n.m.r. spectroscopic data.
    Additional Material: 3 Tab.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1002/prac.19853270309
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  • 10
    Electronic Resource
    Electronic Resource
    Über die Thiocyanierung von AcetylendicarbonsäuredialkylesternI. Mitteilung der Serie „Organische Elektronenleiter und Vorstufen“ (1983)
    New York, NY : Wiley-Blackwell
    Journal für Praktische Chemie/Chemiker-Zeitung 325 (1983), S. 153-156 
    Details
    ISSN: 0021-8383
    Keywords: Chemistry ; Organic Chemistry
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Chemistry and Pharmacology
    Notes: About the Thiocyanation of Dialkyl Acetylendicarboxylates
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1002/prac.19833250119
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