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Methane steam reforming, methanation and water-gas shift: I. Intrinsic kinetics (1989)

Xu, Jianguo ; Froment, Gilbert F.

Hoboken, NJ : Wiley-Blackwell

AIChE Journal 35 (1989), S. 88-96

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ISSN: 0001-1541

Keywords: Chemistry ; Chemical Engineering

Source: Wiley InterScience Backfile Collection 1832-2000

Topics: Chemistry and Pharmacology , Process Engineering, Biotechnology, Nutrition Technology

Notes: Intrinsic rate equations were derived for the steam reforming of methane, accompanied by water-gas shift on a Ni/MgAl2O4 catalyst. A large number of detailed reaction mechanisms were considered. Thermodynamic analysis helped in reducing the number of possible mechanisms. Twenty one sets of three rate equations were retained and subjected to model discrimination and parameter estimation. The parameter estimates in the best model are statistically significant and thermodynamically consistent.

Additional Material: 9 Ill.

Type of Medium: Electronic Resource

URL: http://dx.doi.org/10.1002/aic.690350109

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