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The dynamics of equally spaced multilevel model systems (1991)

Amirav, A. ; Even, U. ; Jortner, Joshua

New York, NY : Wiley-Blackwell

International Journal of Quantum Chemistry 39 (1991), S. 387-397

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Details

ISSN: 0020-7608

Schlagwort(e): Computational Chemistry and Molecular Modeling ; Atomic, Molecular and Optical Physics

Quelle: Wiley InterScience Backfile Collection 1832-2000

Thema: Chemie und Pharmazie

Notizen: Coherent dynamics of multilevel systems is of interest for the elucidation of energy disposal and multiphoton chemistry of polyatomic molecules. We compare the analytical solutions for coherent multiphoton excitation of two sparse multilevel model systems: (1) The spin-J system consisting of N = (2J + 1) equally spaced levels with the radiative coupling being determined by the xth component of the angular momentum. (2) The equally coupled N level system. The transition amplitudes for system (1) are always periodic, which is in contrast to the nonperiodic behavior exhibited by system (2) for N 〉 3.

Zusätzliches Material: 2 Ill.

Materialart: Digitale Medien

URL: http://dx.doi.org/10.1002/qua.560390315

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