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Semiempirical determination of molecular motions associated with phonon modes in molecular crystals (1990)

White, K. M. ; Eckhardt, C. J.

College Park, Md. : American Institute of Physics (AIP)

The Journal of Chemical Physics 92 (1990), S. 2214-2218

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ISSN: 1089-7690

Source: AIP Digital Archive

Topics: Physics , Chemistry and Pharmacology

Notes: An approach using piezomodulated Raman scattering is presented which permits determination of the molecular motions associated with the eigenmodes of molecular crystals. When coupled with a lattice dynamical calculation for the eigenmodes, the experiment can be used to validate the calculation. The case of 1,2,4,5-tetrabromobenzene is treated and it is shown that the phase relations of the piezomodulated Raman signals confirm the calculated eigenmodes.

Type of Medium: Electronic Resource

URL: http://dx.doi.org/10.1063/1.458013

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