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  • Electronic Resource  (2)
  • 2000-2004  (2)
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  • Electronic Resource  (2)
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  • 1
    Electronic Resource
    Electronic Resource
    [S.l.] : American Institute of Physics (AIP)
    Physics of Plasmas 8 (2001), S. 3824-3832 
    ISSN: 1089-7674
    Source: AIP Digital Archive
    Topics: Physics
    Notes: The transport of ground-state hydrogen atoms in the expansion of a thermal hydrogen plasma created by a cascaded arc is studied by means of two-photon absorption laser induced fluorescence. The low-dissociation degree measured at the source exit implies that H atoms flow in a H2 environment. It is shown that the H atom expansion pattern is in disagreement with the neutral gas supersonic expansion theory. Indeed the transport of H atoms in the plasma jet is strongly influenced by surface-recombination processes. Because of the large density gradients between the core of the jet and its surroundings induced by the recombination of H atoms at the reactor walls, hydrogen atoms diffuse out of the plasma jet in the course of the expansion. When the surface loss probability is high, i.e., the combination of a large wall-recombination probability with a long residence time, the losses of radicals by diffusion cannot be avoided even when the mass of the carrier gas is close to the mass of the radical. © 2001 American Institute of Physics.
    Type of Medium: Electronic Resource
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  • 2
    Electronic Resource
    Electronic Resource
    Woodbury, NY : American Institute of Physics (AIP)
    Applied Physics Letters 81 (2002), S. 418-420 
    ISSN: 1077-3118
    Source: AIP Digital Archive
    Topics: Physics
    Notes: The generation of ammonia from atomic hydrogen and nitrogen has been demonstrated by means of cavity enhanced absorption spectroscopy. The atomic species are produced in a thermal plasma source in which plasma is created from mixtures of hydrogen and nitrogen. It is shown that for large atomic flux conditions, 2% of the hydrogen and nitrogen can be converted to ammonia. The process in which the ammonia molecules are formed from atomic radicals at the fully covered surface is called plasma-activated catalysis. © 2002 American Institute of Physics.
    Type of Medium: Electronic Resource
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