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  • 1
    ISSN: 1572-8986
    Keywords: Dielectric barrier discharge ; SO2 removal ; NO removal ; gasphase oxidation
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology , Mechanical Engineering, Materials Science, Production Engineering, Mining and Metallurgy, Traffic Engineering, Precision Mechanics , Technology
    Notes: Abstract A gas-phase oxidation method using dielectric barrier discharges (DBDs) has been developed to remove SO2 and to simultaneously remove SO2 and NO from gas streams that are similar to gas streams generated by the combustion of fossil fuels. SO2 and NO removal efficiencies are evaluated as a function of applied voltage, temperature, and concentrations of SO2, NO, H2O(g), and NH3. With constant H2O(g) concentration, both SO2 and NO removal efficiencies increase with increasing temperature from 100 to 160°C. At 160°C with 15% by volume H20(g), more than 95% of the NO and 32% of the S02 are simultaneously removed from the gas stream. Injection of NH3 into the gas stream caused an increase in S02 removal efficiency to essentially 100%. These results indicate that DBD plasmas have the potential to simultaneously remove SO2 and NO from gas streams generated by large-scale fossil fuel combustors.
    Type of Medium: Electronic Resource
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  • 2
    Electronic Resource
    Electronic Resource
    Springer
    Plasma chemistry and plasma processing 18 (1998), S. 215-239 
    ISSN: 1572-8986
    Keywords: Plasma ; CH4 ; RF ; FTIR ; decomposition ; sensitivity
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology , Mechanical Engineering, Materials Science, Production Engineering, Mining and Metallurgy, Traffic Engineering, Precision Mechanics , Technology
    Notes: Abstract A radio-frequency (RF) plasma system was used to convert methane gas. The reactants and final products were analyzed by using an FTIR (Fourier transform infrared spectrometer). The effects of plasma operational parameters, including feeding concentration (C) of CH 4 , operational pressure (P) in the RF plasma reactor, total gas flow rate (Q) and input power wattage (W) for CH 4 decomposition were evaluated. The results showed that the CH 4 decomposition fraction increases with increasing power input, decreasing operational pressure in the RF plasma reactor, decreasing CH 4 feeding concentration, and decreasing total gas flow rate. In addition, mathematical models based on the obtained experimental data were developed and tested by means of sensitivity analysis.
    Type of Medium: Electronic Resource
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