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  • 1
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: The local magnetic structure of TbFe multilayers with various layer thicknesses of Tb (26 A(ring)) and Fe (10, 20, 30 and 35 A(ring)) has been investigated by circular magnetic x-ray dichroism (CMXD) studies. From the dichroic signal at the L3 edge both the local magnetic Tb moment and the anisotropic behavior of the Tb compound could be deduced. The magnetic spectra at the Tb L2 edge and the Fe K edge, which are known to be sensitive to the local chemical environment, have been used to obtain information on the binding characters of the magnetized atoms in the various TbFe compositions. Significant deviations of the CMXD spectra compared to the corresponding spectra in the pure Fe and Tb metals have been observed. This indicates significant contributions to the magnetism from an interface region, whose chemical structure resembles strongly those of the intermetallic TbFe2 compounds.
    Type of Medium: Electronic Resource
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  • 2
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: Circular magnetic x-ray dichroism (CMXD) was observed at the Pt and Ir L2,3 edges in the multilayered structures 25⋅(4 A(ring) Co+30 A(ring) Pt) and 25⋅(4 A(ring) Co+11 A(ring) Pt+8 A(ring) Ir+11 A(ring) Pt). The samples were prepared by sputtering and show a large perpendicular anisotropy. The magnetic absorption at the Pt and Ir L2,3 edges was measured in an external magnetic field of 0.15 T perpendicular to the surface. The results indicate a significant spin polarization of the Pt and Ir layers. By comparison with the corresponding CMXD signals of Pt and Ir impurities in a ferromagnetic iron host we estimated the local spin and orbital moments. The results show that the innermost three monolayers in both systems couple ferromagnetically to the Co layers with an average magnetic moment of about 0.01 μB.
    Type of Medium: Electronic Resource
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  • 3
    Electronic Resource
    Electronic Resource
    [S.l.] : American Institute of Physics (AIP)
    Journal of Applied Physics 73 (1993), S. 5346-5346 
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: The interference of charge and magnetic scattering from ferromagnetic targets leads in case of circularly polarized x rays to a relative difference (flipping ratio) of the Bragg peak intensity in the order of 10−3, when the magnetization aligned in the scattering plane is reversed (spin-dependent scattering). We have measured the spin-dependent scattering in Fe, Gd, and Tb polycrystalline metallic foils using circularly polarized synchrotron radiation. From the data, magnetic form factors have been deduced. As demonstrated for Gd and Tb, from the flipping ratios the orbital and spin contribution can be directly separated by varying the angle between the scattering vector and the sample magnetization. Spin-dependent resonance scattering has been studied at the K edge of a Ni single crystal. A significant enhancement of the magnetic scattering amplitude compared to the magnetic resonance scattering of linearly polarized light and sample magnetization perpendicular to the scattering plane has been observed. A strongly increased nonresonant magnetic scattering with opposite sign compared to the resonant magnetic effects is observed in the preedge energy region below −10 eV with respect to the K-absorption onset. The applicability of magnetic scattering using circularly polarized synchrotron radiation for the investigation of ferromagnetic media especially in view of its complementarity to neutron studies is discussed.
    Type of Medium: Electronic Resource
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  • 4
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: The method of spin-dependent absorption has been used to examine the temperature dependence of the circular magnetic x-ray dichroism (CMXD) of the (disordered) Invar alloy fcc Fe72Pt28. At the Fe K edge the difference of the transmission for the reversed magnetization direction was determined with an accuracy of 10−5. By comparing the dichroic effects at 110 and at 410 K evidence was found for a temperature-dependent change of the magnetic absorption profile different from the pure amplitude reduction due to the reduced magnetization. It indicates a change of the spin splitting in the low-lying unoccupied p states. The polarization-averaged absorption spectrum shows also a small variation between 4 and 11 eV above the threshold indicating that the p-like electron density drops when the sample is heated. The experimental CMXD profiles are compared with spin-polarized band-structure calculations for ordered Fe3Pt and discussed within the frame of the model of high-spin–low-spin transitions in the Invar regime.
    Type of Medium: Electronic Resource
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  • 5
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: Magnetic circular dichroism (MCD) studies at K and L edges using hard and soft x rays are presented. The relation of this universal phenomenon in the x-ray absorption near-edge structure (XANES) and extended x-ray absorption fine structure (EXAFS) regions to local magnetic structures in the case of 3d and 4f elements is illustrated. The validity of atomic and band-structure pictures to describe the MCD in the XANES range are outlined and the applicability of sum rules and two-step vector coupling models to deduce spin and orbital moments of the absorbing atom as well as spin-density profiles from the experimental data are critically discussed. The correlation of the dichroic contribution in the EXAFS to the magnetic moments and spin densities of the neighboring atoms are addressed by systematic studies which provide new insights into the exchange phenomena of the interaction of spin-polarized electrons with ferromagnetic media. The potential but also the limitations of this new spectroscopy is demonstrated.
    Type of Medium: Electronic Resource
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  • 6
    Electronic Resource
    Electronic Resource
    [S.l.] : American Institute of Physics (AIP)
    Journal of Applied Physics 73 (1993), S. 5347-5347 
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: Systematic studies of the magnetic or spin-dependent EXAFS (SPEXAFS) were performed at the L2/3 edges of Eu3Fe5O12, Gd and Tb metal and the alloy Ho20Gd80. The magnetic absorption exhibits distinct EXAFS structure, more pronounced than the nonmagnetic EXAFS. The Fourier transform of the Eu L2/3-edges SPEXAFS spectra, which are measured with an accuracy of less than 5×10−5, show a complete disappearance of the oxygen peak. This allows an identification of the positions of the magnetic neighbors for a significantly longer range as it is possible by using the conventional EXAFS profile. Studies of the alloy Ho20Gd80 at the L2/3 edges of both components, which show no significant differences in the polarization averaged EXAFS, indicate an essential influence of the spin structure at the absorbing atom on the magnetic EXAFS spectrum. At the L3 edge of Gd and Tb metal (both of hcp structure) we found similar structures in the conventional as well as in the magnetic EXAFS. The data are interpreted in terms of the sensibility of the SPEXAFS on the angular momentum of the absorbing and neighboring atoms.
    Type of Medium: Electronic Resource
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  • 7
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: We have performed systematic investigations of the circular magnetic x-ray dichroism, i.e., the spin-dependent absorption of circularly polarized x rays at the L2,3 edges of the 4f elements in the compound (RE)2Co17. In all systems significant CMXD signals with relative large amplitudes of some percent have been found. It is expected, that the spin-dependent absorption profile reflects the spin-density of d-like unoccupied states at the Fermi level and thus contains information on the orientation of the 4f moment. The ratio of the CMXD signal at the L2 and L3 edges depends strongly on the angular momentum of the 4f core and indicates in case of Ce2Co17, that the 4f electrons are of itinerant character with almost quenched angular momentum, as theoretically expected for similar Ce systems.
    Type of Medium: Electronic Resource
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