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  • 78.70.Dm  (2)
  • 78.20.Ls  (1)
  • PACS. 78.70.Dm X-ray absorption spectra – 71.28.+d Narrow-band systems; intermediate-valence solids – 79.60.-i Photoemission and photoelectron spectra  (1)
Materialart
Erscheinungszeitraum
Schlagwörter
  • 1
    Digitale Medien
    Digitale Medien
    Springer
    Applied physics 60 (1995), S. 179-189 
    ISSN: 1432-0630
    Schlagwort(e): 75.50.Cc ; 78.20.Ls ; 79.60.Cn
    Quelle: Springer Online Journal Archives 1860-2000
    Thema: Maschinenbau , Physik
    Notizen: Abstract 4f Photoemission (PE) spectra from magnetically ordered rare-earth materials using circularly polarized X-rays exhibit strong Magnetic Circular Dichroism (MCD), i.e., the intensities of the individual multiplet lines depend on the relative orientation of sample magnetization and photon spin. On the example of the wellresolved Tb 4f PE multiplet, it is shown that in relevant cases 4f PE lines are essentially only observed for one magnetization direction, either parallel or antiparallel to the photon spin. These large MCD effects in 4f PE open new perspectives in the analysis of surface and thin-film magnetism and provide a sensor for the degree of circular polarization of soft X-rays over a wide photon-energy range. To demonstrate the potential of MCD in 4f PE as a magnetometer, we studied Gd(0001) and Tb(0001), where the magnetization of the topmost atomic (0001) layer can be easily separated from the bulk magnetization via the surface core-level shift. In multicomponent magnetic thin films containing different rare-earth elements 4f PE allows to monitor magnetization in an element-specilic way, e.g., in case of the hetero-magnetic interface 1 ML En/Gd(0001).
    Materialart: Digitale Medien
    Bibliothek Standort Signatur Band/Heft/Jahr Verfügbarkeit
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  • 2
    Digitale Medien
    Digitale Medien
    Springer
    The European physical journal 95 (1994), S. 9-12 
    ISSN: 1434-6036
    Schlagwort(e): 74.70.Vy ; 78.70.Dm ; 79.60.Eq
    Quelle: Springer Online Journal Archives 1860-2000
    Thema: Physik
    Notizen: Abstract Resonant photoemission studies have been performed at the 2p soft-x-ray absorption thresholds of Fe, Co, and Ni metal. At resonance, the photoelectron intensity exhibits a strong enhancement in the region of the two-hole satellites, which is shown, however, to be mostly due to an incoherent superposition of a photoemission signal with a more intense signal from anL 3 M 4,5 M 4,5 Coster-Kronig decay of the core-ionized state. The resonant enhancement of the valence-band photoemission satellite in Ni metal amounts to a factor of ≃12. In contrast, no photoemission satellites are observed for Fe and Co metal.
    Materialart: Digitale Medien
    Bibliothek Standort Signatur Band/Heft/Jahr Verfügbarkeit
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  • 3
    Digitale Medien
    Digitale Medien
    Springer
    The European physical journal 94 (1994), S. 1-2 
    ISSN: 1434-6036
    Schlagwort(e): 79.60.Cn ; 78.70.Dm
    Quelle: Springer Online Journal Archives 1860-2000
    Thema: Physik
    Notizen: Abstract We report on comparative study of angle-resolved photoelectron spectra of Ni metal and CeGd at theM III andN IV,V soft-x-ray absorption threshold, respectively. OnM III resonance, the valence-band photoemission (PE) intensity of Ni follows a cos2-behavior, while the intensity of the 6-eV satellite is independent of the angle of emission relative to the E-vector of the incoming beam. On the other hand, the 4f Ce PE signal behaves ∝ cos2 onN IV,V resonance. This clearly shows that the resonant enhancement of the 6-eV PE satellite of Ni is mainly caused by an incoherent Auger decay and cannot be described as a resonant PE process.
    Materialart: Digitale Medien
    Bibliothek Standort Signatur Band/Heft/Jahr Verfügbarkeit
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  • 4
    ISSN: 1434-6036
    Schlagwort(e): PACS. 78.70.Dm X-ray absorption spectra – 71.28.+d Narrow-band systems; intermediate-valence solids – 79.60.-i Photoemission and photoelectron spectra
    Quelle: Springer Online Journal Archives 1860-2000
    Thema: Physik
    Notizen: Abstract: A strong anisotropic distribution of the holes in Ni 3 d and O 2 p orbitals is observed in the polarization dependent O 1 s and Ni 2 p 3/2 X-ray absorption spectroscopy of the linear-chain nickelate Y2-xCaxBaNiO5 (x = 0, 0.05, 0.1, 0.2), which demonstrates the one-dimensional nature of the electronic state in these compounds. The holes introduced by Ca-doping occupy both O 2 p and Ni 3 d orbitals along the NiO5 chains. By comparing the experimental Ni 2 p 3/2 absorption spectra of Y2-xCaxBaNiO5 to those from charge transfer multiplet calculations we can derive the orbital character of the additional holes to be of ∼60% O2 p and ∼40% Ni 3 d.
    Materialart: Digitale Medien
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