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Determination of dissociation energy for ligand exchange reaction from EXAFS (2001)

Miyanaga, T. ; Sakane, H. ; Watanabe, I.

Chester : International Union of Crystallography (IUCr)

Journal of synchrotron radiation 8 (2001), S. 680-682

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ISSN: 1600-5775

Source: Crystallography Journals Online : IUCR Backfile Archive 1948-2001

Topics: Geosciences , Physics

Notes: EXAFS (extended X-ray absorption fine structure) experiments were performed at several different temperatures for a series of 3d transition metal ions (Cr3+, Fe3+, Fe2+, Ni2+, Co2+, Zn2+) in aqueous solutions. Anharmonic EXAFS analyses, which include up to third order cumulant, were carried out to study on the metal-oxygen bonding potential. According to the model in which the dissociation process is dominant for the ligand-water exchange reaction, the dissociation energy has been first evaluated from EXAFS in solution phase.

Type of Medium: Electronic Resource

URL: http://dx.doi.org/10.1107/S0909049500015934

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