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  • 32.80.Dz  (2)
  • 35.10.F  (2)
  • Penning trap  (2)
  • 21.10.-k  (1)
Material
Years
Keywords
  • 1
    Electronic Resource
    Electronic Resource
    Amsterdam : Elsevier
    International Journal of Mass Spectrometry and Ion Processes 132 (1994), S. 181-191 
    ISSN: 0168-1176
    Keywords: Accumulation ; ICR ; Penning trap ; Quadrupole excitation ; SQUEACE
    Source: Elsevier Journal Backfiles on ScienceDirect 1907 - 2002
    Topics: Chemistry and Pharmacology , Physics
    Type of Medium: Electronic Resource
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  • 2
    Electronic Resource
    Electronic Resource
    Springer
    The European physical journal 321 (1985), S. 537-547 
    ISSN: 1434-601X
    Keywords: 21.10.-k ; 27.80+w ; 31.30.Gs
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract The isotope shift between197Au (stable) and the radioactive Au isotopes190Au,191Au,192Au and193Au were determined by resonance fluorescence spectroscopy in the 6s 2 S 1/2–6p 2 P 1/2.λ=267.6nm line. The unstable Au isotopes were produced at the ISOLDE mass separator at CERN. The nuclei were investigated semi on-line in a resonance vessel, heated to 1,400°C. The results areδν 190,197=−11.12(39) GHz,δν 191,197=−9.67(12) GHz,δν 192,197=−8.32(15) GHz,δν 193,197=−6.29(11) GHz, corresponding to a change of the mean-square charge radius byδ〈r 2〉190,197 =0.261(12) fm2,δ〈r 2〉191,197=0.227(5) fm2,δ〈r 2〉192,197=0.195(5) fm2,δ〈r 2〉193,197 =0.148(4) fm2.
    Type of Medium: Electronic Resource
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  • 3
    ISSN: 1432-0649
    Keywords: 32.30.—r ; 32.80.Rm ; 32.80.Dz ; 35.10.Hn
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract Resonance ionization mass spectroscopic (RIMS) measurements for trace analysis and spectroscopy of 237Np, the ecologically most important isotope of neptunium, are described. The chemical procedure for the separation of neptunium from aqueous samples as well as the preparation of filaments for RIMS are outlined. Several two- and three-step excitation schemes have been investigated in order to find suitable conditions for the sensitive detection of 237Np. Using a three-step, three-color excitation and ionization scheme an overall detection efficiency of 3×10−8 was obtained, resulting in a detection limit of 4×108 atoms (160 fg) of 237Np. The hyperfine structure splittings of the levels under investigation, which influence the detection limit, were measured. A new method to determine the first ionization potential (IP) was applied to neptunium yielding a value of IP=6.2655(2) eV.
    Type of Medium: Electronic Resource
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  • 4
    ISSN: 1432-0630
    Keywords: 07.65.Eh ; 32.70.Fw ; 32.80.Dz
    Source: Springer Online Journal Archives 1860-2000
    Topics: Mechanical Engineering, Materials Science, Production Engineering, Mining and Metallurgy, Traffic Engineering, Precision Mechanics , Physics
    Notes: Abstract Resonance ionization mass spectroscopy (RIMS) and pulsed-laser induced desorption (PLID) have been combined for ultrasensitive detection and spectroscopy of very small samples of refractive elements. The method has been tested and applied to laser spectroscopy of 5×109 atoms (1.5 pg) of195Au (T 1/2= 183d) implanted at the ISOLDE online mass separator with 60 keV into graphite. A pulsed thermal atomic beam was formed by laser desorption with a 10 ns Nd∶Yag laser pulse. Subsequently the atoms were photoionized in a three-colour, three-step resonant excitation to an autoionizing state. The selectivity was enhanced by a time-of-flight measurement of the photo ions. In resonance, one ion was detected per 105 atoms implanted resulting in a gain in detection efficiency by three orders of magnitude in comparison to the use of a continuous atomic beam. In the course of the experiments several unknown autoionizing states were found, and the lifetime of the 6d 2 D 3/2 state of gold was determined to beτ=10.7(6) ns.
    Type of Medium: Electronic Resource
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  • 5
    ISSN: 1434-601X
    Keywords: 21.10 ; 21.60 ; 27.70 ; 27.80 ; 35.10.F
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract The hyperfine structure splitting and the isotope shift in the λ=266 nm transition of Pt isotopes within the mass range 183 ≦A≦ 198 have been determined by Resonance Ionization Mass Spectroscopy (RIMS) in combination with Pulsed-Laser Induced Desorption (PLID). The Pt isotopes were obtained at the on-line isotope separator ISOLDE-3/CERN as daugthers of the primarily produced Hg isotopes. Magnetic moments, quadrupole moments, and changes in the mean-square charge radii are deduced and compared with results of a particle-triaxial rotor model and mean field calculations. Good agreement with experimental data (including nuclear level schemes and transition probabilities) can only be obtained if triaxial shape is admitted. The calculations yield a smooth transition in the shape of odd-A Pt nuclei from a slightly deformed, nearly oblate195Pt via triaxial197-187Pt to a strongly deformed nearly prolate177Pt.
    Type of Medium: Electronic Resource
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  • 6
    ISSN: 1434-6079
    Keywords: 31.30.G ; 31.30.J ; 35.10.F ; 42.65.C
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract The hyperfine structure and isotope shift of221–226Ra and212,214Ra have been measured in the ionic (Ra II) transition 7s 2 S 1/2–7p 2 P 3/2 (λ=381.4 nm). The method of on-line collinear fast-beam laser spectroscopy has been applied using frequency-doubling of cw dye laser radiation in an external ring cavity. The magnetic hyperfine fields are compared with semi-empirical and ab initio calculations. The analysis of the quadrupole splitting by the same method yields the following, improved values of spectroscopic quadrupole moments:Q s (221Ra)=1.978(7)b,Q s (223Ra)=1.254(3)b and the reanalyzed valuesQ s (209Ra)=0.40(2)b,Q s (211Ra)=0.48(2)b,Q s (227Ra)=1.58(3)b,Q s (229Ra)=3.09(4)b with an additional scaling uncertainty of ±5%. Furthermore, theJ-dependence of the isotope shift is analyzed in both Ra II transitions connecting the 7s 2 S 1/2 ground state with the first excited doublet 7p 2 P 1/2 and 7p 2 P 3/2.
    Type of Medium: Electronic Resource
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  • 7
    ISSN: 1572-9540
    Keywords: atomic structure ; mass measurements ; Penning trap
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract The mass of a highly charged ion is the sum of the mass of the nucleus, the mass of the electrons and the electronic binding energies. High accuracy mass measurements on highly charged ions in a sequence of different charge states yield informations on atomic binding energies, i.e., the ionisation potentials. In our contribution we discuss the possibility of determining atomic binding energies of highly charged ions to better than 20 eV via cyclotron frequency measurements in a Penning trap. At this level of accuracy different contributions to the binding energies, like relativistic corrections, Breit corrections and QED corrections, can be measured.
    Type of Medium: Electronic Resource
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