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  • 31.30.Gs  (3)
  • 32.80.Dz  (2)
  • 1
    Electronic Resource
    Electronic Resource
    Springer
    The European physical journal 321 (1985), S. 537-547 
    ISSN: 1434-601X
    Keywords: 21.10.-k ; 27.80+w ; 31.30.Gs
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract The isotope shift between197Au (stable) and the radioactive Au isotopes190Au,191Au,192Au and193Au were determined by resonance fluorescence spectroscopy in the 6s 2 S 1/2–6p 2 P 1/2.λ=267.6nm line. The unstable Au isotopes were produced at the ISOLDE mass separator at CERN. The nuclei were investigated semi on-line in a resonance vessel, heated to 1,400°C. The results areδν 190,197=−11.12(39) GHz,δν 191,197=−9.67(12) GHz,δν 192,197=−8.32(15) GHz,δν 193,197=−6.29(11) GHz, corresponding to a change of the mean-square charge radius byδ〈r 2〉190,197 =0.261(12) fm2,δ〈r 2〉191,197=0.227(5) fm2,δ〈r 2〉192,197=0.195(5) fm2,δ〈r 2〉193,197 =0.148(4) fm2.
    Type of Medium: Electronic Resource
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  • 2
    ISSN: 1432-0630
    Keywords: 07.65.Eh ; 32.70.Fw ; 32.80.Dz
    Source: Springer Online Journal Archives 1860-2000
    Topics: Mechanical Engineering, Materials Science, Production Engineering, Mining and Metallurgy, Traffic Engineering, Precision Mechanics , Physics
    Notes: Abstract Resonance ionization mass spectroscopy (RIMS) and pulsed-laser induced desorption (PLID) have been combined for ultrasensitive detection and spectroscopy of very small samples of refractive elements. The method has been tested and applied to laser spectroscopy of 5×109 atoms (1.5 pg) of195Au (T 1/2= 183d) implanted at the ISOLDE online mass separator with 60 keV into graphite. A pulsed thermal atomic beam was formed by laser desorption with a 10 ns Nd∶Yag laser pulse. Subsequently the atoms were photoionized in a three-colour, three-step resonant excitation to an autoionizing state. The selectivity was enhanced by a time-of-flight measurement of the photo ions. In resonance, one ion was detected per 105 atoms implanted resulting in a gain in detection efficiency by three orders of magnitude in comparison to the use of a continuous atomic beam. In the course of the experiments several unknown autoionizing states were found, and the lifetime of the 6d 2 D 3/2 state of gold was determined to beτ=10.7(6) ns.
    Type of Medium: Electronic Resource
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  • 3
    ISSN: 1432-0649
    Keywords: 32.30.—r ; 32.80.Rm ; 32.80.Dz ; 35.10.Hn
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract Resonance ionization mass spectroscopic (RIMS) measurements for trace analysis and spectroscopy of 237Np, the ecologically most important isotope of neptunium, are described. The chemical procedure for the separation of neptunium from aqueous samples as well as the preparation of filaments for RIMS are outlined. Several two- and three-step excitation schemes have been investigated in order to find suitable conditions for the sensitive detection of 237Np. Using a three-step, three-color excitation and ionization scheme an overall detection efficiency of 3×10−8 was obtained, resulting in a detection limit of 4×108 atoms (160 fg) of 237Np. The hyperfine structure splittings of the levels under investigation, which influence the detection limit, were measured. A new method to determine the first ionization potential (IP) was applied to neptunium yielding a value of IP=6.2655(2) eV.
    Type of Medium: Electronic Resource
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  • 4
    Electronic Resource
    Electronic Resource
    Springer
    The European physical journal 7 (1987), S. 193-201 
    ISSN: 1434-6079
    Keywords: 31.30.Gs ; 35.10.Fk
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract Isotope shift (IS) and hyperfine structure (hfs) measurements have been performed on seven lines of the platinum I spectrum with interference as well as laser fluorescence spectroscopy. In the latter case a frequency-doubled single-mode cw dye laser was applied. The IS of190Pt with a natural abundance of only 0.01% was determined to beδν 190, 192=−38.65(8) mK in theλ306.47 nm transition. The IS parameters and the effective hfs integrals in the configuration (5d+6s)10 were determined in intermediate coupling by a least squares fit of the IS and hfs data with eigenvectors obtained from the platinum fine structure (fs). The results are compared with theoretical values and yield improvedδ〈r 2〉 data.
    Type of Medium: Electronic Resource
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  • 5
    ISSN: 1434-6079
    Keywords: 31.30.Gs ; 31.50. + w ; 35.10.Fk
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract The hyperfine spectra of the 5s4d 3 D 1-5s20f, 5s4d 3 D 2-5s23f, and 5s 4d 3 D 3-5s32f transitions of87Sr (I=9/2) have been measured by collinear fast beam laser spectroscopy. The structure in the upper configurations is highly perturbed by fine structure splitting that is of comparable size to the hyperfine interaction energy. These perturbations can be adequately treated with conventional matrix diagonalization methods, using the 5s-electron magnetic dipole interaction terma 5s and the unperturbed fine structure splittings as input parameters. Additionally, hyperfine constants for the lower 5s4d 3 D configurations, including theA- andB-factors and a separation of the individuals- andd-electron contributions to these factors, are derived.
    Type of Medium: Electronic Resource
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