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  • 1
    ISSN: 1434-601X
    Keywords: 23.60.+e ; 25.70.−z ; 27.80.+w
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract New neutron-deficient isotopes,197Rn,197mRn, and200Fr have been produced and identified on the basis of genetic correlations in the166Er(36Ar,5n)197Rn (Elab=186, 200 MeV), and169Tm(36Ar,5n)200Fr (Elab=186 MeV) reactions. The evaporation residues were separated from the beam by using a gas-filled recoil separator and implanted onto a position-sensitive solid-state detector. The α-decay energies (half-lives) of197Rn,197mRn and200Fr have been determined to be 7261±30 keV (51 −15 +35 ms), 7370±30 keV (18 −5 +9 ms), and 7500±3O keV, (570 −140 +270 ms), respectively.
    Type of Medium: Electronic Resource
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  • 2
    ISSN: 1434-601X
    Keywords: PACS:25.85.-w Fission reactions – 25.85.Ge Charged-particle-induced fission
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract: Angular distributions of fission fragments with mass number A=97-159 have been measured by the radiochemical recoil-catcher method in the proton-induced fission of 244Pu with the incident energy of 15 MeV. Angular anisotropies of extreme asymmetric mass division products even up to the fragment mass ratio of A H /A L ∼ 1.85 are found not any different from those of the typical asymmetric mass division products with A∼ 138, which indicates that no clear evidence is observed for the existence of an additional saddle point configuration in the extreme asymmetric mass division. The correlation between the saddle point state evaluated from the angular anisotropy and the mass division mode is discussed.
    Type of Medium: Electronic Resource
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  • 3
    Electronic Resource
    Electronic Resource
    Springer
    Journal of radioanalytical and nuclear chemistry 234 (1998), S. 95-100 
    ISSN: 1588-2780
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology , Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The stability of 16 kinds of metallofullerenes (9 elements) was investigated against the recoil phenomena associated with the capture of neutrons by the metal atoms inside the carbon cages. The yields of the unaffected species were obtained by use of the HPLC separation method and radioactivity measurements. Recoil energy distributions of the metal atoms were calculated theoretically and the effective energy required for destruction of metallofullerenes from inside by recoiling atoms was estimated to be about 10 to 15 eV for the metallofullerenes containing lanthanide atoms.
    Type of Medium: Electronic Resource
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  • 4
    Electronic Resource
    Electronic Resource
    Springer
    Journal of radioanalytical and nuclear chemistry 234 (1998), S. 27-32 
    ISSN: 1588-2780
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology , Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Nondestructive determination of major and trace elements within voluminous materials has been demonstrated by prompt γ-ray neutron activation analysis. Some fragmented pieces of pottery bowls considered to have been produced in the late 18th century were analyzed by a new internal monostandard method, and noticeable differences of the elemental contents and significant correlations of the elemental distributions were observed among the samples. The possibility of identification of producing areas of unearthened material is demonstrated by the analytical results and the applicability of this method to the investigation of precious samples in a completely nondestructive way is verified in practice.
    Type of Medium: Electronic Resource
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  • 5
    Electronic Resource
    Electronic Resource
    Springer
    Journal of radioanalytical and nuclear chemistry 239 (1999), S. 179-185 
    ISSN: 1588-2780
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology , Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The effect of β−-decay on the stability of metallofullerenes was investigated for three decay chains of155Sm-155Eu,161Gd-161Tb and177Yb-177Lu. For the former two cases, the metallofullerenes were found stable even after the β−-decay while in the case of177Yb, the metallofullerene became unstable after β−-decay. The present results point to the fact that metallofullerenes are stable against ordinary β−-decay unstable after β−-decay. The present results point to the fact that metallofullerenes are stable against ordinary β−-decay recoil energies, but they become unstable if the oxidation state of the metal atom is changed by nuclear transformation.
    Type of Medium: Electronic Resource
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  • 6
    Electronic Resource
    Electronic Resource
    Springer
    Journal of radioanalytical and nuclear chemistry 192 (1995), S. 81-89 
    ISSN: 1588-2780
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology , Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Advantages and uniqueness of radiochemical techniques in fullerene studies are pointed out. Some experimental data are presented on metallofullerenes production yields, HPLC elution behaviors of Y, La, Gd containing fullerenes, encapsulation of a new metal in the carbon cage, stability of the carbon cage against recoil energy, and the distribution of metallofullerenes among various organs of rats.
    Type of Medium: Electronic Resource
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  • 7
    Electronic Resource
    Electronic Resource
    Springer
    Journal of radioanalytical and nuclear chemistry 239 (1999), S. 365-369 
    ISSN: 1588-2780
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology , Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Fullerenes, C60 and C70, were irradiated by 8 and 10 MeV deuterons. The irradiated samples were dissolved in CS2 and filtered to remove insoluble by-products. Finally, radioactive fullerenes and products, such as fullerene dimers, trimers labeled with13N, were isolated and detected in the liquid phase by radiochromatography. This suggests that the energy rich13N atoms successfully incorporated into the fullerene cages and that the disrupted cages reacted with neighboring cages.
    Type of Medium: Electronic Resource
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  • 8
    Electronic Resource
    Electronic Resource
    Springer
    Journal of radioanalytical and nuclear chemistry 239 (1999), S. 581-585 
    ISSN: 1588-2780
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology , Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Prompt γ-ray analysis using the internal monostandard method was applied to voluminous archaeological bronze mirrors produced in ancient China. Sn/Cu content ratios were determined nondestructively by this method. Furthermore, Au/Cu, As/Cu, and Sb/Cu content ratios were determined by means of measuring decay γ-rays emitted from radioactive nuclides produced within samples via (n,γ) reactions. It is clear that the Sn/Cu content ratios in bronze mirrors produced in the Sung era is smaller than in ones produced in between the Han and the Tung era.
    Type of Medium: Electronic Resource
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  • 9
    Electronic Resource
    Electronic Resource
    Springer
    Journal of radioanalytical and nuclear chemistry 239 (1999), S. 187-190 
    ISSN: 1588-2780
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology , Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Time-differential perturbed angular correlation method was applied to Ce@C82 in order to investigate the electronic properties of the encaged Ce atom. The nuclear quadrupole frequency of the nuclear spin of the Ce was successfully determined as ωQ = 6.5(3)·107 rad/s, which is much greater than what has already been estimated for Ce4+ and La3+ in other compounds. By comparing the present value with the values for the Ce4+ and La3+, it was inferred that the valence state of the encaged Ce atom is trivalent.
    Type of Medium: Electronic Resource
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  • 10
    Electronic Resource
    Electronic Resource
    Springer
    Journal of radioanalytical and nuclear chemistry 239 (1999), S. 201-206 
    ISSN: 1588-2780
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology , Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The11C and14C labeled fullerenes were produced by charged-particle and neutron irradiation, of C60, C70 and their mixture. It was found that a carbon atom of fullerence can be easily exchanged with a radioactive carbon atom produced by a nuclear reaction. The HPLC method was effective for identification and purification of various labeled fullerene families as chemically stable compounds. The radiochemically interesting aspect of the results is not only the production of11C and14C labeled fullerenes but also the formation of radioactive higher fullerenes which can be simultaneously produced with high yield and in carrier-free form.
    Type of Medium: Electronic Resource
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