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  • 35.10.Fk  (3)
  • 32.70.Fw  (2)
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  • 1
    ISSN: 1432-0630
    Keywords: 07.65.Eh ; 32.70.Fw ; 32.80.Dz
    Source: Springer Online Journal Archives 1860-2000
    Topics: Mechanical Engineering, Materials Science, Production Engineering, Mining and Metallurgy, Traffic Engineering, Precision Mechanics , Physics
    Notes: Abstract Resonance ionization mass spectroscopy (RIMS) and pulsed-laser induced desorption (PLID) have been combined for ultrasensitive detection and spectroscopy of very small samples of refractive elements. The method has been tested and applied to laser spectroscopy of 5×109 atoms (1.5 pg) of195Au (T 1/2= 183d) implanted at the ISOLDE online mass separator with 60 keV into graphite. A pulsed thermal atomic beam was formed by laser desorption with a 10 ns Nd∶Yag laser pulse. Subsequently the atoms were photoionized in a three-colour, three-step resonant excitation to an autoionizing state. The selectivity was enhanced by a time-of-flight measurement of the photo ions. In resonance, one ion was detected per 105 atoms implanted resulting in a gain in detection efficiency by three orders of magnitude in comparison to the use of a continuous atomic beam. In the course of the experiments several unknown autoionizing states were found, and the lifetime of the 6d 2 D 3/2 state of gold was determined to beτ=10.7(6) ns.
    Type of Medium: Electronic Resource
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  • 2
    ISSN: 1434-601X
    Keywords: 21.10.Ft ; 21.10.ky ; 35.10.Fk
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract The technique of collinear fast-beam laser spectroscopy has been used to measure the isotope shifts of the even-even isotopes of Hg (Z=80) in the mass range 182≤A≤198 at the on-line mass separator ISOLDE at CERN. The atomic transition studied (6s 6p 3 P 2- 6s7s 3 S 1,λ=546.1 nm) starts from a metastable state, which is populated in a quasi resonant charge transfer process. The resulting changes in nuclear mean square charge radii show clearly that182Hg follows the trend of the heavier, even, weakly oblate isotopes. Correspondingly the huge odd-even shape staggering in the light Hg isotopes continues and the nuclear shape staggering and shape coexistence persists down to the last isotope investigated,181Hg. An update of isotope shift and hyperfine structure data for181–206Hg is given, with a revised evaluation of the differences in nuclear mean square charge radii and of spectroscopic quadrupole moments.
    Type of Medium: Electronic Resource
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  • 3
    Electronic Resource
    Electronic Resource
    Springer
    The European physical journal 7 (1987), S. 193-201 
    ISSN: 1434-6079
    Keywords: 31.30.Gs ; 35.10.Fk
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract Isotope shift (IS) and hyperfine structure (hfs) measurements have been performed on seven lines of the platinum I spectrum with interference as well as laser fluorescence spectroscopy. In the latter case a frequency-doubled single-mode cw dye laser was applied. The IS of190Pt with a natural abundance of only 0.01% was determined to beδν 190, 192=−38.65(8) mK in theλ306.47 nm transition. The IS parameters and the effective hfs integrals in the configuration (5d+6s)10 were determined in intermediate coupling by a least squares fit of the IS and hfs data with eigenvectors obtained from the platinum fine structure (fs). The results are compared with theoretical values and yield improvedδ〈r 2〉 data.
    Type of Medium: Electronic Resource
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  • 4
    ISSN: 1434-6079
    Keywords: 32.70.Fw ; 32.80.Rm
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract Lifetimes of Rydberg states of the triplet-series 5s ns 3 S 1 withn = 19–23, 35 and 5s nd 3 D 3 withn = 18–20, 23–28 in the spectrum of neutral strontium have been determined. Observation of the exponential decay after excitation by a pulsed laser in a fast atomic beam and subsequent state-selective field ionization was employed. The lifetimes of the states of the3 S 1-series show the expectedn*3 dependence on the effective principal quantum number, while the3 D 3-series is disturbed by configuration mixing. Furthermore, state re-populations induced by black-body radiation have been observed.
    Type of Medium: Electronic Resource
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  • 5
    ISSN: 1434-6079
    Keywords: 31.30.Gs ; 31.50. + w ; 35.10.Fk
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract The hyperfine spectra of the 5s4d 3 D 1-5s20f, 5s4d 3 D 2-5s23f, and 5s 4d 3 D 3-5s32f transitions of87Sr (I=9/2) have been measured by collinear fast beam laser spectroscopy. The structure in the upper configurations is highly perturbed by fine structure splitting that is of comparable size to the hyperfine interaction energy. These perturbations can be adequately treated with conventional matrix diagonalization methods, using the 5s-electron magnetic dipole interaction terma 5s and the unperturbed fine structure splittings as input parameters. Additionally, hyperfine constants for the lower 5s4d 3 D configurations, including theA- andB-factors and a separation of the individuals- andd-electron contributions to these factors, are derived.
    Type of Medium: Electronic Resource
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